Scanning internal photoemission microscopy for the identification of hot carrier transport mechanisms

被引:5
作者
Differt, D. [1 ]
Pfeiffer, W. [1 ]
Diesing, D. [2 ]
机构
[1] Univ Bielefeld, Fak Phys, D-33615 Bielefeld, Germany
[2] Univ Duisburg Essen, Fak Chem, D-45117 Essen, Germany
关键词
INSULATOR-METAL JUNCTIONS; EXCITED ELECTRONS; RELAXATION; EMISSION; DYNAMICS; GAS;
D O I
10.1063/1.4752734
中图分类号
O59 [应用物理学];
学科分类号
摘要
Linear and nonlinear internal photoemission in a thin-film metal-insulator-metal heterosystem, i.e., a Ta-TaOx-Ag junction, together with surface reflectivity are mapped with a lateral resolution of better than 5 mu m. The spatial correlation of the different signals and time-resolved internal photoemission spectroscopy reveal excitation mechanisms and ballistic hot carrier injection. The internal photoemission yield variation with Ag layer thickness is quantitatively explained by above-barrier injection. The hot-spot-like behavior of the two-photon induced internal photoemission observed for short pulse excitation is attributed to local field enhancements because of Ag-film thickness reduction and plasmonic effects at structural defects. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4752734]
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页数:4
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