Hydrogen production methods efficiency coupled to an advanced high-temperature accelerator driven system

被引:7
作者
Rodriguez, Daniel Gonzalez [1 ]
Brayner de Oliveira Lira, Carlos Alberto [2 ]
Garcia Hernandez, Carlos Rafael [3 ]
de Andrade Lima, Fernando Roberto [1 ]
机构
[1] Ctr Reg Ciencias Nucl Nordeste CRCN NE, Ave Prof Luiz Freire 1000, BR-50740535 Recife, PE, Brazil
[2] Univ Fed Pernambuco, Dept Energia Nucl, Ave Prof Luiz Freire 1000, BR-50740535 Recife, PE, Brazil
[3] Inst Super Tecnol & Ciencias Aplicadas InSTEC CUB, Ave Salvador Allende Esq, Havana 10400, Cuba
关键词
Nuclear hydrogen production; ADS; HTE; Sulfur-iodine; Efficiency; Cost estimative; MULTIPHASE BUNSEN REACTION; SOLID OXIDE ELECTROLYSIS; SULFUR-IODINE CYCLE; THERMOCHEMICAL CYCLE; H2SO4; DECOMPOSITION; PART I; ENERGY; MODEL; EQUATION; REACTORS;
D O I
10.1016/j.ijhydene.2018.11.083
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Hydrogen, rather than oil, must be produced in volumes not provided by the currently employed methods. In this work, two high-temperature hydrogen production methods coupled with an advanced nuclear system are presented. A new design of a pebble-bed accelerator nuclear-driven system called TADSEA (Transmutation Advanced Device for Sustainable Energy Applications) was chosen because of the advantages in transmutation and safety. A detailed flowsheet of the high-temperature electrolysis process coupled to TADSEA through a Brayton gas cycle was developed using chemical process simulation software: Aspen HYSYS (R). It is obtained 0.1627 kg/s of hydrogen with the model with optimized operating conditions, resulting in an overall process efficiency of 34.51%, a value in the range of results reported by other authors. A conceptual design of a plant using the iodine-sulfur thermochemical water splitting cycle was carried out producing 5.66e-2 kg/s and electric energy in cogeneration. The overall efficiency was calculated performing an energy balance resulting in 22.56%. A brief hydrogen production cost estimation was performed for both methods obtaining 5.96$/kg for the sulfur-iodine (SI) and 4.8 $/kg for the high-temperature electrolysis (HTE) process. (C) 2018 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:1392 / 1408
页数:17
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