Robustness of Basal-Plane Antiferromagnetic Order and the Jeff=1/2 State in Single-Layer Iridate Spin-Orbit Mott Insulators

被引:112
作者
Boseggia, S. [1 ,3 ]
Springell, R. [4 ]
Walker, H. C. [5 ]
Ronnow, H. M. [6 ]
Rueegg, Ch. [7 ,8 ]
Okabe, H. [9 ]
Isobe, M. [9 ]
Perry, R. S. [10 ]
Collins, S. P. [3 ]
McMorrow, D. F. [1 ,2 ]
机构
[1] UCL, London Ctr Nanotechnol, London WC1E 6BT, England
[2] UCL, Dept Phys & Astron, London WC1E 6BT, England
[3] Diamond Light Source Ltd, Didcot OX11 0DE, Oxon, England
[4] Univ Bristol, Interface Anal Ctr, Royal Commiss Exhibit Res Fellow 1851, Bristol BS2 8BS, Avon, England
[5] Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany
[6] Ecole Polytech Fed Lausanne, ICMP, Lab Quantum Magnetism, CH-1015 Lausanne, Switzerland
[7] Paul Scherrer Inst, Neutron Scattering Lab, CH-5232 Villigen, Switzerland
[8] Univ Geneva, DPMC MaNEP, CH-1211 Geneva, Switzerland
[9] Natl Inst Mat Sci, Tsukuba, Ibaraki 3050044, Japan
[10] Univ Edinburgh, Sch Phys, Scottish Univ Phys Alliance, Edinburgh EH9 3JZ, Midlothian, Scotland
基金
英国工程与自然科学研究理事会;
关键词
HIGH-TEMPERATURE SUPERCONDUCTIVITY; SR2IRO4; PHYSICS;
D O I
10.1103/PhysRevLett.110.117207
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The magnetic structure and electronic ground state of the layered perovskite Ba2IrO4 have been investigated using x-ray resonant magnetic scattering. Our results are compared with those for Sr2IrO4, for which we provide supplementary data on its magnetic structure. We find that the dominant, long-range antiferromagnetic order is remarkably similar in the two compounds and that the electronic ground state in Ba2IrO4, deduced from an investigation of the x-ray resonant magnetic scattering L-3/L-2 intensity ratio, is consistent with a J(eff) = 1/2 description. The robustness of these two key electronic properties to the considerable structural differences between the Ba and Sr analogues is discussed in terms of the enhanced role of the spin-orbit interaction in 5d transition metal oxides. DOI: 10.1103/PhysRevLett.110.117207
引用
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页数:5
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