Single-photon multiple ionization forming double vacancies in the 2p subshell of argon

被引:12
作者
Linusson, P. [1 ]
Fritzsche, S. [2 ,3 ]
Eland, J. H. D. [4 ,5 ]
Mucke, M. [5 ]
Feifel, R. [5 ]
机构
[1] Stockholm Univ, AlbaNova Univ Ctr, Dept Phys, SE-10691 Stockholm, Sweden
[2] Helmholtz Inst Jena, D-07743 Jena, Germany
[3] Univ Jena, Inst Theoret Phys, D-07743 Jena, Germany
[4] Univ Oxford, Dept Chem, Phys & Theoret Chem Lab, Oxford OX1 3QZ, England
[5] Uppsala Univ, Dept Phys & Astron, SE-75120 Uppsala, Sweden
来源
PHYSICAL REVIEW A | 2013年 / 87卷 / 04期
基金
瑞典研究理事会;
关键词
DIFFERENTIAL CROSS-SECTIONS; OPEN-SHELL ATOMS; DOUBLE PHOTOIONIZATION; AUGER; SPECTRUM; HELIUM; XENON;
D O I
10.1103/PhysRevA.87.043409
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Single-photon ionization leading to two vacancies in the 2p subshell of argon is investigated experimentally using the photoelectron time-of-flight magnetic bottle coincidence technique. Three peaks corresponding to the P-3, D-1, and S-1 states of the dication are found in the ionization energy range 535 to 562 eV. Multiconfigurational Dirac-Fock calculations were performed to estimate the single-photon double-ionization cross sections. Reasonable agreement between the measured and simulated spectra is found if single and double excitations are taken into account in the wave-function expansion. DOI: 10.1103/PhysRevA.87.043409
引用
收藏
页数:6
相关论文
共 38 条
[1]   Formation of Kr3+ via core-valence doubly ionized intermediate states [J].
Andersson, E. ;
Linusson, P. ;
Fritzsche, S. ;
Hedin, L. ;
Eland, J. H. D. ;
Karlsson, L. ;
Rubensson, J. -E. ;
Feifel, R. .
PHYSICAL REVIEW A, 2012, 85 (03)
[2]   Single-photon core-valence double ionization of molecular oxygen [J].
Andersson, E. ;
Stenrup, M. ;
Eland, J. H. D. ;
Hedin, L. ;
Berglund, M. ;
Karlsson, L. ;
Larson, A. ;
Agren, H. ;
Rubensson, J. -E. ;
Feifel, R. .
PHYSICAL REVIEW A, 2008, 78 (02)
[3]   ARGON KLL AND KLM AUGER-ELECTRON SPECTRA [J].
ASPLUND, L ;
KELFVE, P ;
BLOMSTER, B ;
SIEGBAHN, H ;
SIEGBAHN, K .
PHYSICA SCRIPTA, 1977, 16 (5-6) :268-272
[4]   A study of Ne2+ and Ar2+ satellite states observed by 'threshold photoelectrons coincidence' spectroscopy [J].
Avaldi, L ;
Dawber, G ;
Gulley, N ;
Rojas, H ;
King, GC ;
Hall, R ;
Stuhec, M ;
Zitnik, M .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1997, 30 (22) :5197-5212
[5]   Photo-double-ionization of atoms [J].
Bolognesi, P ;
King, GC ;
Avaldi, L .
RADIATION PHYSICS AND CHEMISTRY, 2004, 70 (1-3) :207-236
[6]   OBSERVATION OF K HYPERSATELLITES AND KL SATELLITES IN X-RAY SPECTRUM OF DOUBLY K-IONIZED GALLIUM [J].
BRIAND, JP ;
CHEVALLIER, P ;
TAVERNIER, M ;
ROZET, JP .
PHYSICAL REVIEW LETTERS, 1971, 27 (12) :777-+
[7]   Xenon N4,5OO Auger spectrum -: a useful calibration source [J].
Carroll, TX ;
Bozek, JD ;
Kukk, E ;
Myrseth, V ;
Sæthre, LJ ;
Thomas, TD ;
Wiesner, K .
JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA, 2002, 125 (02) :127-132
[8]   Fully quantal (γ, 2e) calculations for absolute differential cross sections of helium [J].
Colgan, J ;
Pindzola, MS ;
Robicheaux, F .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2001, 34 (15) :L457-L466
[9]   Double Core Hole Creation and Subsequent Auger Decay in NH3 and CH4 Molecules [J].
Eland, J. H. D. ;
Tashiro, M. ;
Linusson, P. ;
Ehara, M. ;
Ueda, K. ;
Feifel, R. .
PHYSICAL REVIEW LETTERS, 2010, 105 (21)
[10]   Complete two-electron spectra in double photoionization: The rare gases Ar, Kr, and Xe [J].
Eland, JHD ;
Vieuxmaire, O ;
Kinugawa, T ;
Lablanquie, P ;
Hall, RI ;
Penent, F .
PHYSICAL REVIEW LETTERS, 2003, 90 (05) :4