Gas-phase single-shot thermometry at 1 kHz using fs-CARS spectroscopy

被引:74
作者
Roy, Sukesh [1 ]
Kulatilaka, Waruna D. [1 ]
Richardson, Daniel R. [2 ]
Lucht, Robert P. [2 ]
Gord, James R. [3 ]
机构
[1] Spectral Energies LLC, Dayton, OH 45431 USA
[2] Purdue Univ, Sch Mech Engn, W Lafayette, IN 47907 USA
[3] USAF, Res Lab, Prop Directorate, Wright Patterson AFB, OH 45433 USA
基金
美国国家科学基金会;
关键词
FEMTOSECOND CARS;
D O I
10.1364/OL.34.003857
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Single-laser-shot temperature measurements at a data rate of 1 kHz employing femtosecond coherent anti-Stokes Raman scattering (fs-CARS) spectroscopy of N(2) are demonstrated. The measurements are performed using a chirped-probe pulse to map the time-dependent frequency-spread dephasing of the Raman coherence, which is created by similar to 80-fs pump and Stokes beams, into the spectrum of the coherent anti-Stokes Raman scattering signal pulse. Temperature is determined from the spectral shape of the fs-CARS signal for probe delays of similar to 2 ps with respect to the pump-Stokes excitation. The accuracy and precision of the measurements for the 300-2400 K range are found to be similar to 1%-6% and similar to 1.5%-3%, respectively. (C) 2009 Optical Society of America
引用
收藏
页码:3857 / 3859
页数:3
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