Suppression of the long-range magnetic order in Pb3(Mn1-xFex)7O15 upon substitution of Fe for Mn

被引:4
作者
Volkov, N. V. [1 ]
Eremin, E. V. [1 ]
Bayukov, O. A. [1 ]
Sablina, K. A. [1 ]
Solov'ev, L. A. [2 ]
Velikanov, D. A. [1 ]
Mikhashenok, N. V. [1 ]
Osetrov, E. I. [1 ]
Schefer, J. [3 ,4 ]
Keller, L. [3 ,4 ]
Boehm, M. [5 ]
机构
[1] Russian Acad Sci, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
[2] Russian Acad Sci, Siberian Branch, Inst Chem & Chem Technol, Krasnoyarsk 660046, Russia
[3] ETH, Neutron Scattering Lab, CH-5232 Villigen, Switzerland
[4] Paul Scherrer Inst, CH-5232 Villigen, Switzerland
[5] Inst Max Von Laue Paul Langevin, F-38042 Grenoble 9, France
关键词
Crystal growth; Ferrimagnetism; Layered magnetic compounds; PROFILE REFINEMENT; PB3MN7O15;
D O I
10.1016/j.jmmm.2013.04.054
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Structure and magnetic properties of Pb-3(Mn1-xFex)(7)O-15 single crystals with x=0-0.2 grown by spontaneous crystallization from solution in melt have been investigated. All the crystals belong to the hexagonal space group P6(3)/mcm. The magnetic properties appeared to be strongly dependent on the iron doping level. At small (x=0.05) dopant concentrations, the value of magnetization and Neel temperature T-N decrease insignificantly (T-N=70 K). With increasing x, the three-dimensional magnetic ordering does not occur and temperature dependences of magnetization at x >= 0.1 exhibit spin-glass-like features in the low-temperature region. (c) 2013 Elsevier B.V. All rights reserved.
引用
收藏
页码:100 / 107
页数:8
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