Key results from irradiation and post-irradiation examination of AGR-1 UCO TRISO fuel

被引:41
作者
Demkowicz, Paul A. [1 ]
Hunn, John D. [2 ]
Petti, David A. [1 ]
Morris, Robert N. [2 ]
机构
[1] Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA
[2] Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA
关键词
TRISO; AGR-1; UCO; Fuel irradiation; Post-irradiation examination; Fuel performance; COATED PARTICLE FUEL; TEMPERATURE REACTOR-FUEL; GAS-COOLED REACTORS; SILVER; COMPACTS; IDENTIFICATION; PERFORMANCE; PALLADIUM; RELEASE; CESIUM;
D O I
10.1016/j.nucengdes.2017.09.005
中图分类号
TL [原子能技术]; O571 [原子核物理学];
学科分类号
0827 ; 082701 ;
摘要
The AGR-1 irradiation experiment was performed as the first test of tristructural isotropic (TRISO) fuel in the US Advanced Gas Reactor Fuel Development and Qualification Program. The experiment consisted of 72 right cylinder fuel compacts containing approximately 3 x 10(5) coated fuel particles with uranium oxide/uranium carbide (UCO) fuel kernels. The fuel was irradiated in the Advanced Test Reactor for a total of 620 effective full power days. Fuel burnup ranged from 11.3 to 19.6% fissions per initial metal atom and time-average, volumeaverage irradiation temperatures of the individual compacts ranged from 955 to 1136 degrees C. This paper focuses on key results from the irradiation and post-irradiation examination, which revealed a robust fuel with excellent performance characteristics under the conditions tested and have significantly improved the understanding of UCO coated particle fuel irradiation behavior. The fuel exhibited zero TRISO coating failures (failure of all three dense coating layers) during irradiation and post-irradiation safety testing at temperatures up to 1700 degrees C. Advanced PIE methods have allowed particles with SiC coating failure that were discovered to be present in a very-low population to be isolated and meticulously examined, which has elucidated the specific causes of SiC failure in these specimens. The level of fission product release from the fuel during irradiation and post-irradiation safety testing has been studied in detail. Results indicated very low release of krypton and cesium through intact SiC and modest release of europium and strontium, while also confirming the potential for significant silver release through the coatings depending on irradiation conditions. Focused study of fission products within the coating layers of irradiated particles down to nanometer length scales has provided new insights into fission product transport through the coating layers and the role various fission products may have on coating integrity. The broader implications of these results and the application of lessons learned from AGR-1 to fuel fabrication and post-irradiation examination for subsequent fuel irradiation experiments as part of the US fuel program are also discussed.
引用
收藏
页码:102 / 109
页数:8
相关论文
共 36 条
[1]   DIFFUSION OF SILVER AND CESIUM IN SILICON-CARBIDE COATINGS OF FUEL-PARTICLES FOR HIGH-TEMPERATURE GAS-COOLED REACTORS [J].
AMIAN, W ;
STOVER, D .
NUCLEAR TECHNOLOGY, 1983, 61 (03) :475-486
[2]  
[Anonymous], 2006, ORNLCF0602
[3]  
Collin B.P., 2015, Tech. Rep. INL/EXT-10-18097 Rev. 3
[4]   Comparison of silver, cesium, and strontium release predictions using PARFUME with results from the AGR-1 irradiation experiment [J].
Collin, Blaise P. ;
Petti, David A. ;
Demkowicz, Paul A. ;
Maki, John T. .
JOURNAL OF NUCLEAR MATERIALS, 2015, 466 :426-442
[5]  
Demkowicz P.A., 2015, Tech. Rep. INL/EXT-15-36407
[6]  
Demkowicz P. A., 2013, 13 28483 INLEXT
[7]   Irradiation performance of AGR-1 high temperature reactor fuel [J].
Demkowicz, Paul A. ;
Hunn, John D. ;
Ploger, Scott A. ;
Morris, Robert N. ;
Baldwin, Charles A. ;
Harp, Jason M. ;
Winston, Philip L. ;
Gerczak, Tyler J. ;
van Rooyen, Isabella J. ;
Montgomery, Fred C. ;
Silva, Chinthaka M. .
NUCLEAR ENGINEERING AND DESIGN, 2016, 306 :2-13
[8]   First high temperature safety tests of AGR-1 TRISO fuel with the Fuel Accident Condition Simulator (FACS) furnace [J].
Demkowicz, Paul A. ;
Reber, Edward L. ;
Scates, Dawn M. ;
Scott, Les ;
Collin, Blaise P. .
JOURNAL OF NUCLEAR MATERIALS, 2015, 464 :320-330
[9]   Accident testing of high-temperature reactor fuel elements from the HFR-EU1bis irradiation [J].
Freis, D. ;
Bottomley, P. D. W. ;
Kellerbauer, A. I. ;
Rondinella, V. V. ;
Van Uffelen, P. .
NUCLEAR ENGINEERING AND DESIGN, 2011, 241 (08) :2813-2821
[10]  
Gerczak T. J., 2016, J NUCL MATER, V480, P1