A Facile Synthesis of Nitrogen-Doped Porous Carbon Materials for High-Performance Supercapacitors

被引:8
作者
Yao, Lu [1 ]
Chen, Da-Ming [1 ]
Yan, Song [1 ]
Lin, Jing-Jing [1 ]
Liu, Ye-Ping [1 ]
Lian, Jun [1 ]
Liu, Yue-Ran [1 ]
Lin, Hua-Lin [1 ]
Han, Sheng [1 ]
机构
[1] Shanghai Inst Technol, Sch Chem & Environm Engn, Haiquan Rd 100, Shanghai 201418, Peoples R China
来源
CHEMISTRYSELECT | 2019年 / 4卷 / 09期
基金
中国国家自然科学基金;
关键词
N-doping; supercapacitor; melamine; foam; freestanding; carbon; material; SUPERIOR PERFORMANCE; ACTIVATED CARBON; CO2; CAPTURE; ELECTRODE; BIOMASS; SPHERES; POLYANILINE; NANOTUBES; TEMPLATE; NETWORKS;
D O I
10.1002/slct.201803808
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A simple way for N-doped porous carbon materials (ANCs) was prepared in N-2 atmosphere through the KOH-assisted carbonization of commercial melamine foam (MF) attached glucose. Adding glucose and KOH activation process have great effects on improving the electrochemical properties of ANCs materials. Compared with other materials, the optimal ANCs-800, which is obtained with a KOH/glucose/MF weight ratio of 5:20:1 at 800 degrees C, exhibits the best capacitance performance with the specific surface area (SSA) of 1481 m(2 )g(-1) and high nitrogen content of 3.7 at. %. It possesses prominent specific capacitance (387 F g(-1) at 0.5 A g(-1) ) and excellent cycling stability (98.6% retention after 10,000 cycles). Furthermore, in the symmetric supercapacitor, the ANCs-800 electrode material maintains high energy density (24.2 W h kg(-1) at 701.07 W kg(-1)) and great cycling performance (96.3% after 10,000 cycles). Accordingly, the facile synthetic approach and attractive electrochemical properties make ANCs-800 a popular capacitor material.
引用
收藏
页码:2726 / 2733
页数:8
相关论文
共 47 条
  • [1] Nitrogen-doped activated carbons derived from a co-polymer for high supercapacitor performance
    Alabadi, Akram
    Yang, Xinjia
    Dong, Zehua
    Li, Zhen
    Tan, Bien
    [J]. JOURNAL OF MATERIALS CHEMISTRY A, 2014, 2 (30) : 11697 - 11705
  • [2] Free-standing fluorine and nitrogen co-doped graphene paper as a high-performance electrode for flexible sodium-ion batteries
    An, Haoran
    Li, Yu
    Gao, Yi
    Cao, Chen
    Han, Junkai
    Feng, Yiyu
    Feng, Wei
    [J]. CARBON, 2017, 116 : 338 - 346
  • [3] Nitrogen-Doped Carbon Coated Stainless Steel Meshes for Flexible Supercapacitors
    Cao, Jing
    Huang, Tao
    Liu, Ruili
    Xi, Xin
    Wu, Dongqing
    [J]. ELECTROCHIMICA ACTA, 2017, 230 : 265 - 270
  • [4] N/P co-doped hierarchical porous carbon materials for superior performance supercapacitors
    Chen, Jing
    Wei, Huanming
    Chen, Haijun
    Yao, Wenhao
    Lin, Hualin
    Han, Sheng
    [J]. ELECTROCHIMICA ACTA, 2018, 271 : 49 - 57
  • [5] Nitrogen-doped hierarchically porous carbon foam: A free-standing electrode and mechanical support for high-performance supercapacitors
    Chen, Jizhang
    Xu, Junling
    Zhou, Shuang
    Zhao, Ni
    Wong, Ching-Ping
    [J]. NANO ENERGY, 2016, 25 : 193 - 202
  • [6] Nitrogen-doped porous carbon for supercapacitor with long-term electrochemical stability
    Chen, Xiang Ying
    Chen, Chong
    Zhang, Zhong Jie
    Xie, Dong Hua
    Deng, Xiao
    Liu, Jian Wei
    [J]. JOURNAL OF POWER SOURCES, 2013, 230 : 50 - 58
  • [7] How Do Pseudocapacitors Store Energy? Theoretical Analysis and Experimental Illustration
    Costentin, Cyrille
    Porter, Thomas R.
    Saveant, Jean-Michel
    [J]. ACS APPLIED MATERIALS & INTERFACES, 2017, 9 (10) : 8649 - 8658
  • [8] Assembly of graphene aerogels into the 3D biomass-derived carbon frameworks on conductive substrates for flexible supercapacitors
    Fan, Ya-Meng
    Song, Wei-Li
    Li, Xiaogang
    Fan, Li-Zhen
    [J]. CARBON, 2017, 111 : 658 - 666
  • [9] Recycling the biowaste to produce nitrogen and sulfur self-doped porous carbon as an efficient catalyst for oxygen reduction reaction
    Gao, Shuyan
    Li, Lingyu
    Geng, Keran
    Wei, Xianjun
    Zhang, Shuxia
    [J]. NANO ENERGY, 2015, 16 : 408 - 418
  • [10] Foldable supercapacitors from triple networks of macroporous cellulose fibers, single-walled carbon nanotubes and polyaniline nanoribbons
    Ge, Dengteng
    Yang, Lili
    Fan, Lei
    Zhang, Chuanfang
    Xiao, Xu
    Gogotsi, Yury
    Yang, Shu
    [J]. NANO ENERGY, 2015, 11 : 568 - 578