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Photovoltage from ferroelectric domain walls in BiFeO3
被引:9
|作者:
Korbel, Sabine
[1
,2
]
Sanvito, Stefano
[1
,2
]
机构:
[1] Trinity Coll Dublin, Sch Phys, AMBER, Dublin 2, Ireland
[2] Trinity Coll Dublin, CRANN Inst, Dublin 2, Ireland
基金:
欧盟地平线“2020”;
爱尔兰科学基金会;
关键词:
CRYSTAL;
TEMPERATURE;
EXCITONS;
OXIDE;
D O I:
10.1103/PhysRevB.102.081304
中图分类号:
T [工业技术];
学科分类号:
08 ;
摘要:
We calculate the component of the photovoltage in bismuth ferrite that is generated by ferroelectric domain walls, using first-principles methods, in order to compare its magnitude to the experimentally measured photovoltage. We find that excitons at the ferroelectric domain walls form an electric dipole layer resulting in a domain-wall driven photovoltage. This is of the same order of magnitude as the experimentally measured one, but only if the carrier lifetimes and diffusion lengths are larger than previously assumed.
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页数:7
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