Tracking emission rate dynamics of nitrogen vacancy centers in nanodiamonds

被引：18
|
作者：
Inam, F. A. [1 ,2 ,3 ]
Edmonds, A. M. [1 ,2 ,3 ]
Steel, M. J. [1 ,2 ]
Castelletto, S. [1 ,2 ,3 ]
机构：
[1] Macquarie Univ, Dept Phys & Astron, MQ Photon Res Ctr, N Ryde, NSW 2109, Australia
[2] Macquarie Univ, Dept Phys & Astron, Ctr Quantum Sci & Technol, N Ryde, NSW 2109, Australia
[3] Macquarie Univ, Dept Phys & Astron, ARC Ctr Excellence Engn Quantum Syst EQuS, N Ryde, NSW 2109, Australia
来源：
APPLIED PHYSICS LETTERS | 2013年 / 102卷 / 25期
关键词：
NV CENTERS; DIAMOND; MICROSCOPY; SPIN;
D O I：
10.1063/1.4812711
中图分类号：
O59 [应用物理学];
学科分类号：
摘要：
Spontaneous emission from crystal centers is influenced by both the photonic local density of states and non-radiative processes. Here, we monitor the spontaneous emission of single nitrogen vacancy (NV) centers as their host diamond is reduced in size from a large monolithic crystal to a nanocrystal by successive cycles of oxidation. The size reduction induces a quenching of the NV radiative emission. Additional non-radiative channels lead to a decrease of the fluorescence intensity and the excited state lifetime. In one case, we observe the onset of blinking which may provide a route to understand these additional non-radiative decay channels. (C) 2013 AIP Publishing LLC.
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页数：5
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