Oxidative Coupling of Methane: Optimal Operating Policies for a Membrane Reactor Network

被引:4
|
作者
Lenhart, Eva [1 ]
Esche, Erik [1 ]
Arellano-Garcia, Harvey [1 ]
Biegler, Lorenz T. [2 ]
机构
[1] Tech Univ Berlin, Fachgebiet Dynam & Betrieb Tech Anlagen, D-10623 Berlin, Germany
[2] Carnegie Mellon Univ, Dept Chem Engn, Pittsburgh, PA 15213 USA
关键词
Membrane reactor network; Oxidative coupling of methane; Packed-bed membrane reactor; Process optimization; LA2O3/CAO CATALYST;
D O I
10.1002/cite.201200073
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
The oxidative coupling of methane (OCM), in which methane is turned into ethylene and ethane, presents an opportunity for using natural gas to produce desired C2 hydrocarbons. The main challenge for the successful implementation of the process is the reduction of undesired by-products, such as CO2. This contribution deals with the optimization of a membrane reactor network for the OCM process with the goal of maximizing yield while maintaining simultaneously a high selectivity in C2 products. The network consists of a plug flow/fixed-bed reactor, a conventional packed-bed membrane reactor and a so-called proposed packed-bed membrane reactor.
引用
收藏
页码:1980 / 1988
页数:9
相关论文
共 50 条
  • [41] Oxidative Coupling of Methane: A Comparison of Different Reactor Configurations
    Cruellas, Aitor
    Melchiori, Tommaso
    Gallucci, Fausto
    Annaland, Martin van Sint
    ENERGY TECHNOLOGY, 2020, 8 (08)
  • [42] Inorganic membrane reactors for the oxidative coupling of methane
    Tonkovich, ALY
    Jimenez, DM
    Zilka, JL
    Roberts, GL
    CHEMICAL ENGINEERING SCIENCE, 1996, 51 (11) : 3051 - 3056
  • [43] Analysis of oxidative coupling of methane in membrane reactors
    Godini, H. R.
    Arellano-Garcia, H.
    Omidkhah, M. R.
    Wozny, G.
    19TH EUROPEAN SYMPOSIUM ON COMPUTER AIDED PROCESS ENGINEERING, 2009, 26 : 123 - 128
  • [44] Recognition of Oxidative Coupling of Methane Reactor Performance Patterns
    Kim, Mijin
    Repke, Jens-Uwe
    Schomäcker, Reinhard
    Khodadadi, Abbas Ali
    Wozny, Günter
    Görke, Oliver
    Godini, Hamid Reza
    Chemical Engineering and Technology, 2022, 45 (04): : 694 - 708
  • [45] Optimization of fluidized bed reactor of oxidative coupling of methane
    Eghbal-Ahmadi, Mohammad-Hosein
    Zaerpour, Masoud
    Daneshpayeh, Mahdi
    Mostoufi, Navid
    International Journal of Chemical Reactor Engineering, 2012, 10 (01)
  • [46] PULSE REACTOR STUDIES OF CATALYSTS FOR THE OXIDATIVE COUPLING OF METHANE
    DAHL, IM
    JENS, KJ
    SLAGTERN, A
    CATALYSIS TODAY, 1992, 13 (2-3) : 345 - 352
  • [47] Recognition of Oxidative Coupling of Methane Reactor Performance Patterns
    Kim, Mijin
    Repke, Jens-Uwe
    Schomaecker, Reinhard
    Khodadadi, Abbas Ali
    Wozny, Guenter
    Goerke, Oliver
    Godini, Hamid Reza
    CHEMICAL ENGINEERING & TECHNOLOGY, 2022, 45 (04) : 694 - 708
  • [48] Perovskite-type ceramic membrane: synthesis, oxygen permeation and membrane reactor performance for oxidative coupling of methane
    Zeng, Y
    Lin, YS
    Swartz, SL
    JOURNAL OF MEMBRANE SCIENCE, 1998, 150 (01) : 87 - 98
  • [49] Inorganic membrane reactors for the oxidative coupling of methane
    Pacific Northwest Natl Lab, Richland, United States
    Chemical Engineering Science, 1996, 51 (11 pt B): : 3051 - 3056
  • [50] Perovskite-type ceramic membrane: Synthesis, oxygen permeation and membrane reactor performance for oxidative coupling of methane
    Department of Chemical Engineering, University of Cincinnati, Cincinnati, OH 45221-0171, United States
    不详
    J. Membr. Sci., 1 (87-98):