Evaluation of proton transport and solvation effect in hydrated Nafion membrane with degradation

被引:8
作者
Hu, Yu [1 ]
Wang, Shuai [1 ]
He, Yurong [1 ]
An, Liang [2 ]
机构
[1] Harbin Inst Technol, Sch Energy Sci & Engn, Harbin 150001, Peoples R China
[2] Hong Kong Polytech Univ, Dept Mech Engn, Hung Hom, Hong Kong, Peoples R China
关键词
MOLECULAR-DYNAMICS SIMULATIONS; WATER-SORPTION; MODEL;
D O I
10.1039/d2cp02817d
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In proton exchange membrane fuel cells (PEMFCs), free radicals easily attack ionomers, resulting in membrane degradation. In this work, the multistate empirical valence bond (MS-EVB) method is employed to investigate the chemical degradation impact of Nafion membranes on proton transport and the solvation effect. The hydrophilic domain and its connectivity are analyzed. The numbers of surrounding water and hydronium ions as well as the location of the solvation shell are evaluated. The results demonstrate that the membrane degradation does not change the interaction with the hydronium ions and water molecules but alters the coordination number, leading to a larger hydrophilic domain and a poorer connectivity. The acid groups and protons are distributed more at the edge of the hydrophilic region to accelerate the proton motion, which is not conducive to the proton transport along the membrane side chain.
引用
收藏
页码:29024 / 29033
页数:10
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