A giant magnetoresistance effect (similar to 46% at 20K under 7 T) and anomalous magnetic properties were found in a highly epitaxial double perovskite LaBaCo2O5.5+delta (LBCO) thin film on (001) MgO. Aberration-corrected Electron Microscopy and related analytical techniques were employed to understand the nature of these unusual physical properties. The as-grown film is epitaxial with the c-axis of the LBCO structure lying in the film plane and with an interface relationship given by (100)(LBCO) || (001)(MgO) and [001](LBCO) || [100](MgO) or [010](MgO). Orderly oxygen vacancies were observed by line profile electron energy loss spectroscopy and by atomic resolution imaging. Especially, oxygen vacancy and nanodomain structures were found to have a crucial effect on the electronic transport and magnetic properties. (C) 2014 AIP Publishing LLC.
机构:
Bhabha Atom Res Ctr, Beamline Dev & Applicat Sect, Mumbai 400085, India
Homi Bhabha Natl Inst, Mumbai 400094, IndiaBhabha Atom Res Ctr, Beamline Dev & Applicat Sect, Mumbai 400085, India
Nand, Mangla
Tripathi, Shilpa
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Bhabha Atom Res Ctr, Beamline Dev & Applicat Sect, Mumbai 400085, IndiaBhabha Atom Res Ctr, Beamline Dev & Applicat Sect, Mumbai 400085, India
Tripathi, Shilpa
Rajput, Parasmani
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Bhabha Atom Res Ctr, Beamline Dev & Applicat Sect, Mumbai 400085, IndiaBhabha Atom Res Ctr, Beamline Dev & Applicat Sect, Mumbai 400085, India
Rajput, Parasmani
Kumar, Manvendra
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Shri Vaishnav Vidyapeeth Vishwavidyalaya, Inst Sci, Dept Phys, Indore 453111, IndiaBhabha Atom Res Ctr, Beamline Dev & Applicat Sect, Mumbai 400085, India
Kumar, Manvendra
Kumar, Yogesh
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Bhabha Atom Res Ctr, Beamline Dev & Applicat Sect, Mumbai 400085, IndiaBhabha Atom Res Ctr, Beamline Dev & Applicat Sect, Mumbai 400085, India
Kumar, Yogesh
Mandal, Satish K.
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Saha Inst Nucl Phys Kolkata, Surface Phys & Mat Sci Div, 1-AF Bidhannagar,Sect 1, Kolkata 700064, India
Raja Ramanna Ctr Adv Technol, Accelerator Phys & Synchrotrons Utilizat Devis, Indore 452013, IndiaBhabha Atom Res Ctr, Beamline Dev & Applicat Sect, Mumbai 400085, India
Mandal, Satish K.
Urkude, Rajashri
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Saha Inst Nucl Phys Kolkata, Surface Phys & Mat Sci Div, 1-AF Bidhannagar,Sect 1, Kolkata 700064, India
Raja Ramanna Ctr Adv Technol, Accelerator Phys & Synchrotrons Utilizat Devis, Indore 452013, IndiaBhabha Atom Res Ctr, Beamline Dev & Applicat Sect, Mumbai 400085, India
Urkude, Rajashri
Gupta, Mukul
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UGC, DAE Consortium Sci Res, Univ Campus,Khandwa Rd, Indore 452017, IndiaBhabha Atom Res Ctr, Beamline Dev & Applicat Sect, Mumbai 400085, India
Gupta, Mukul
Dawar, Anit
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Inter Univ Accelerator Ctr, Aruna Asaf Ali Marg, New Delhi 110067, IndiaBhabha Atom Res Ctr, Beamline Dev & Applicat Sect, Mumbai 400085, India
Dawar, Anit
Ojha, Sunil
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Inter Univ Accelerator Ctr, Aruna Asaf Ali Marg, New Delhi 110067, IndiaBhabha Atom Res Ctr, Beamline Dev & Applicat Sect, Mumbai 400085, India
Ojha, Sunil
Rai, S. K.
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Raja Ramanna Ctr Adv Technol, Accelerator Phys & Synchrotrons Utilizat Devis, Indore 452013, IndiaBhabha Atom Res Ctr, Beamline Dev & Applicat Sect, Mumbai 400085, India
Rai, S. K.
Jha, S. N.
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Bhabha Atom Res Ctr, Beamline Dev & Applicat Sect, Mumbai 400085, India
Homi Bhabha Natl Inst, Mumbai 400094, IndiaBhabha Atom Res Ctr, Beamline Dev & Applicat Sect, Mumbai 400085, India
机构:
Indiana Univ, Dept Phys, Bloomington, IN 47405 USAIndiana Univ, Dept Phys, Bloomington, IN 47405 USA
Yang, W. C.
Xie, Y. T.
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Virginia Tech, Dept Phys, Blacksburg, VA 24061 USAIndiana Univ, Dept Phys, Bloomington, IN 47405 USA
Xie, Y. T.
Zhu, W. K.
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Indiana Univ, Dept Phys, Bloomington, IN 47405 USAIndiana Univ, Dept Phys, Bloomington, IN 47405 USA
Zhu, W. K.
Park, K.
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Virginia Tech, Dept Phys, Blacksburg, VA 24061 USAIndiana Univ, Dept Phys, Bloomington, IN 47405 USA
Park, K.
Chen, A. P.
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Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USAIndiana Univ, Dept Phys, Bloomington, IN 47405 USA
Chen, A. P.
Losovyj, Y.
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Indiana Univ, Dept Chem, Bloomington, IN 47405 USAIndiana Univ, Dept Phys, Bloomington, IN 47405 USA
Losovyj, Y.
Li, Z.
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Indiana Univ, Dept Phys, Bloomington, IN 47405 USA
Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USAIndiana Univ, Dept Phys, Bloomington, IN 47405 USA
Li, Z.
Liu, H. M.
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Indiana Univ, Dept Phys, Bloomington, IN 47405 USAIndiana Univ, Dept Phys, Bloomington, IN 47405 USA
Liu, H. M.
Starr, M.
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Indiana Univ, Dept Phys, Bloomington, IN 47405 USAIndiana Univ, Dept Phys, Bloomington, IN 47405 USA
Starr, M.
Acosta, J. A.
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Indiana Univ, Dept Phys, Bloomington, IN 47405 USAIndiana Univ, Dept Phys, Bloomington, IN 47405 USA
Acosta, J. A.
Tao, C. G.
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Virginia Tech, Dept Phys, Blacksburg, VA 24061 USAIndiana Univ, Dept Phys, Bloomington, IN 47405 USA
Tao, C. G.
Li, N.
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Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USAIndiana Univ, Dept Phys, Bloomington, IN 47405 USA
Li, N.
Jia, Q. X.
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Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA
SUNY Buffalo, Dept Mat Design & Innovat, Univ Buffalo, Buffalo, NY 14260 USAIndiana Univ, Dept Phys, Bloomington, IN 47405 USA
Jia, Q. X.
Heremans, J. J.
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Virginia Tech, Dept Phys, Blacksburg, VA 24061 USAIndiana Univ, Dept Phys, Bloomington, IN 47405 USA
Heremans, J. J.
Zhang, S. X.
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Indiana Univ, Dept Phys, Bloomington, IN 47405 USAIndiana Univ, Dept Phys, Bloomington, IN 47405 USA
机构:
Hubei Univ, Fac Phys & Elect Technol, Wuhan 430062, Peoples R China
Tohoku Univ, Inst Mat Res, Sendai, Miyagi 9808577, JapanHubei Univ, Fac Phys & Elect Technol, Wuhan 430062, Peoples R China
Yang, F. J.
Chen, X. Q.
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Hubei Univ, Fac Phys & Elect Technol, Wuhan 430062, Peoples R ChinaHubei Univ, Fac Phys & Elect Technol, Wuhan 430062, Peoples R China