Antimicrobial Dye-Conjugated Polyglobalide-Based Organogels

被引：12
作者：
Rowley, Jason, V [1 ]
Wall, Patrick [1 ]
Yu, Huayang [1 ]
Tronci, Giuseppe [2 ,3 ]
Devine, Deirdre A. [4 ]
Vernon, Jonathan J. [4 ]
Thornton, Paul D. [1 ]
机构：
[1] Univ Leeds, Sch Chem, Leeds LS2 9JT, W Yorkshire, England
[2] Univ Leeds, Sch Dent, Biomat & Tissue Engn Res Grp, St Jamess Univ Hosp, Leeds LS9 7TF, W Yorkshire, England
[3] Univ Leeds, Sch Design, Clothworkers Ctr Text Mat Innovat Healthcare, Leeds LS9 7TF, W Yorkshire, England
[4] Univ Leeds, Sch Dent, Div Oral Biol, Leeds LS2 9JT, W Yorkshire, England
来源：
ACS APPLIED POLYMER MATERIALS | 2020年 / 2卷 / 07期
基金：
英国工程与自然科学研究理事会;
关键词：
antimicrobial organogels; natural oil-based gels; polyester coloration; fragrance release; polyglobalide; ENE CROSS-LINKING; RING-OPENING POLYMERIZATION; DRUG-DELIVERY; SUNFLOWER-OIL; MACROLACTONES; BIODEGRADATION; DEGRADATION; POLYESTERS; BIGELS;
D O I：
10.1021/acsapm.0c00422
中图分类号：
T [工业技术];
学科分类号：
08 ;
摘要：
The straightforward coloration of polyglobalide by the covalent grafting of thiol-modified disperse dyes to afford a colored polyester is reported. The colored polymer could form physical organogels, and upon covalently cross-linking chemical organogels in a range of food-grade oils, and the fragrant and antimicrobial molecule 2-phenylethanol. Antimicrobial testing of the 2-phenylethanol-swollen chemical organogels revealed considerable antimicrobial activity against both Staphylococcus aureus and Escherichia coli. The materials reported offer a range of potential applications, particularly as simple and cost-effective antimicrobial gels.
引用
收藏
页码：2927 / 2933
页数：7
相关论文
共 41 条
[1]   Side-chain functionalisation of unsaturated polyesters from ring-opening polymerisation of macrolactones by thiol-ene click chemistry [J].
Ates, Zeliha ;
Thornton, Paul D. ;
Heise, Andreas .
POLYMER CHEMISTRY, 2011, 2 (02) :309-312
[2]   Functional films from unsaturated poly(macrolactones) by thiol-ene cross-linking and functionalisation [J].
Ates, Zeliha ;
Heise, Andreas .
POLYMER CHEMISTRY, 2014, 5 (08) :2936-2941
[3]   An overview of polylactides as packaging materials [J].
Auras, R ;
Harte, B ;
Selke, S .
MACROMOLECULAR BIOSCIENCE, 2004, 4 (09) :835-864
[4]   Functional biodegradable polymers via ring-opening polymerization of monomers without protective groups [J].
Becker, Greta ;
Wurm, Frederik R. .
CHEMICAL SOCIETY REVIEWS, 2018, 47 (20) :7739-7782
[5]   Modulating the physical properties of sunflower oil and sorbitan monopalmitate-based organogels [J].
Behera, Beauty ;
Sagiri, Sai S. ;
Pal, Kunal ;
Srivastava, Anand .
JOURNAL OF APPLIED POLYMER SCIENCE, 2013, 127 (06) :4910-4917
[6]   Enzymatic degradation of poly (butylene succinate-co-hexamethylene succinate) [J].
Bi, Siwen ;
Tan, Bin ;
Soule, James L. ;
Sobkowicz, Margaret J. .
POLYMER DEGRADATION AND STABILITY, 2018, 155 :9-14
[7]   Self-assembly and multifunctionality of peptide organogels: oil spill recovery, dye absorption and synthesis of conducting biomaterials [J].
Chetia, Monikha ;
Debnath, Swapna ;
Chowdhury, Sumit ;
Chatterjee, Sunanda .
RSC ADVANCES, 2020, 10 (09) :5220-5233
[8]   Photoinduced Thiol-Ene Crosslinking of Globalide/ε-Caprolactone Copolymers: Curing Performance and Resulting Thermoset Properties [J].
Claudino, Mauro ;
van der Meulen, Inge ;
Trey, Stacy ;
Jonsson, Mats ;
Heise, Andreas ;
Johansson, Mats .
JOURNAL OF POLYMER SCIENCE PART A-POLYMER CHEMISTRY, 2012, 50 (01) :16-24
[9]   Biocompatibility, biodegradation and excretion of polylactic acid (PLA) in medical implants and theranostic systems [J].
da Silva, Dana ;
Kaduri, Maya ;
Poley, Maria ;
Adir, Omer ;
Krinsky, Nitzan ;
Shainsky-Roitman, Janna ;
Schroeder, Avi .
CHEMICAL ENGINEERING JOURNAL, 2018, 340 :9-14
[10]   A novel flunarizine hydrochloride-loaded organogel for intraocular drug delivery in situ: Design, physicochemical characteristics and inspection [J].
Dai, Manman ;
Bai, Luyu ;
Zhang, Huimin ;
Ma, Qun ;
Luo, Rui ;
Lei, Fang ;
Fei, Qingsong ;
He, Ning .
INTERNATIONAL JOURNAL OF PHARMACEUTICS, 2020, 576
12345