Fabrication of ternary GO/g-C3N4/MoS2 flower-like heterojunctions with enhanced photocatalytic activity for water remediation

被引:189
作者
Wu, Ming-hong [1 ]
Li, Lin [1 ]
Xue, Yuan-cheng [1 ]
Xu, Gang [2 ]
Tang, Liang [1 ]
Liu, Ning [2 ]
Huang, Wen-yuan [2 ]
机构
[1] Shanghai Univ, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China
[2] Univ Shanghai Sci & Technol, Sch Environm & Architecture, Shanghai 200093, Peoples R China
基金
中国国家自然科学基金;
关键词
Nanocomposite; Surfactant-assisted synthesis; Photocatalysis; Organic dyes; Cr(VI); HYDROGEN-EVOLUTION; MOS2; NANOPARTICLES; NITRIDE NANOSHEETS; ORGANIC FRAMEWORKS; EFFICIENT; GRAPHENE; REDUCTION; COMPOSITE; CHALLENGES; OXIDATION;
D O I
10.1016/j.apcatb.2018.01.063
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
It is extremely important to design excellent nanojunction to improve photocatalytic performance. In this study, we use a simple method to construct GO/g-C3N4/MoS2 ternary-layered nanostructures as an effective photo catalyst for environmental purification using solar energy. The as-prepared materials have more adsorption sites and response sites due to the dual effects of NMP and CTAB. With the visible light irradiation, it has great photodegradation performance for MB, RhB and CV, as well as the photocatalytic reduction ability to Cr (VI). Meanwhile, the nanocomposites exhibit good reproducibility and stability during the cycle of the experiment. The designed heterostructures have a flower structure, which effectively improves the collection of electrons in MoS2 and holes in g-C3N4, effectively reducing the binding of photogenerated electron carriers. Furthermore, GO acts as a fast transport holes, which is attributed to superior its electrical conductivity. This work provides a new field of view for establishing high-efficient and easy-made photocatalysts with environmental remediation.
引用
收藏
页码:103 / 112
页数:10
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