Long-range atmospheric transport of particulate Polycyclic Aromatic Hydrocarbons and the incursion of aerosols to the southeast Tibetan Plateau

被引:54
|
作者
Wang, Xiaoping [1 ,2 ]
Gong, Ping [1 ,2 ]
Sheng, Jiujiang [1 ]
Joswiak, Daniel R. [1 ]
Yao, Tandong [1 ,2 ]
机构
[1] Chinese Acad Sci, Key Lab Tibetan Environm Changes & Land Surface P, Inst Tibetan Plateau Res, Beijing 100101, Peoples R China
[2] CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing, Peoples R China
基金
中国国家自然科学基金;
关键词
Polycyclic Aromatic Hydrocarbons; Tibetan Plateau; Westerly winds; Himalayas; BLACK CARBON; ORGANOCHLORINE PESTICIDES; OPTICAL-PROPERTIES; SOURCE REGIONS; SOURCE APPORTIONMENT; SPATIAL-DISTRIBUTION; EMISSION INVENTORY; BROWN CLOUDS; PAHS; AIR;
D O I
10.1016/j.atmosenv.2015.04.050
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The long range atmospheric transport of Polycyclic Aromatic Hydrocarbons (PAHs) from heavily polluted regions to remote areas has been well-known. However, there are limited studies focussing on the Tibetan Plateau (TP). To assess the temporal transport patterns of PAHs and particulate matters (PMs), a ground-based observation program (2008-2011) was conducted in the southeast TP. Relatively high atmospheric concentrations of particulate-PAHs (0.2-5.0 ng m(-3), sum of 15 compounds) and Total suspended Particles (TSP, 4.1-46.7 mu g m(-3)) were observed. Concentrations of particulate-PAHsITSP exhibited seasonality with higher levels in the winter spring season and lower levels in summer. Using the potential source contribution function model, the source region of both particulate-PAHs and particles was attributed to the Indo-Gangetic Plain (IGP), suggesting the co-transport of particulate-PAHs and aerosols. The aerosol incursion, penetrating the Himalayas and reaching the TP was further captured by Moderate Resolution Imaging Spectroradiometer and Cloud-Aerosol Lidar Infrared Pathfinder Satellite Observations. (C) 2015 Elsevier Ltd. All rights reserved.
引用
收藏
页码:124 / 131
页数:8
相关论文
共 50 条
  • [1] Implications for long-range atmospheric transport of polycyclic aromatic hydrocarbons in Lhasa, China
    Ma, Wan-Li
    Qi, Hong
    Baidron, Sonam
    Liu, Li-Yan
    Yang, Meng
    Li, Yi-Fan
    ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH, 2013, 20 (08) : 5525 - 5533
  • [2] Implications for long-range atmospheric transport of polycyclic aromatic hydrocarbons in Lhasa, China
    Wan-Li Ma
    Hong Qi
    Sonam Baidron
    Li-Yan Liu
    Meng Yang
    Yi-Fan Li
    Environmental Science and Pollution Research, 2013, 20 : 5525 - 5533
  • [3] Dechloranes in lichens from the southeast Tibetan Plateau: Evidence of long-range atmospheric transport
    Yang, Ruiqiang
    Zhang, Shujuan
    Li, Xinghong
    Luo, Dongxia
    Jing, Chuanyong
    CHEMOSPHERE, 2016, 144 : 446 - 451
  • [4] Long-range transport of atmospheric microplastics deposited onto glacier in southeast Tibetan Plateau
    Wang, Zhaoqing
    Zhang, Yulan
    Kang, Shichang
    Yang, Ling
    Luo, Xi
    Chen, Pengfei
    Guo, Junming
    Hu, Zhaofu
    Yang, Chengde
    Yang, Zhengzheng
    Gao, Tanguang
    ENVIRONMENTAL POLLUTION, 2022, 306
  • [5] Long-range atmospheric transport and the distribution of polycyclic aromatic hydrocarbons in Changbai Mountain
    Zhao, Xiangai
    Kim, Seung-Kyu
    Zhu, Weihong
    Kannan, Narayanan
    Li, Donghao
    CHEMOSPHERE, 2015, 119 : 289 - 294
  • [6] Atmospheric particulate polycyclic aromatic hydrocarbons from road transport in southeast Brazil
    Allen, A. G.
    da Rocha, G. O.
    Cardoso, A. A.
    Paterlini, W. C.
    Machado, C. M. D.
    de Andrade, J. B.
    TRANSPORTATION RESEARCH PART D-TRANSPORT AND ENVIRONMENT, 2008, 13 (08) : 483 - 490
  • [7] Seasonal variation and sources of atmospheric polycyclic aromatic hydrocarbons in a background site on the Tibetan Plateau
    Wu, Xuemei
    Sun, Weijun
    Huai, Baojuan
    Wang, Lei
    Han, Chuntan
    Wang, Yetang
    Mi, Wenying
    JOURNAL OF ENVIRONMENTAL SCIENCES, 2023, 125 : 524 - 532
  • [8] Composition and sources of polycyclic aromatic hydrocarbons in cryoconites of the Tibetan Plateau glaciers
    Li, Quanlian
    Kang, Shichang
    Wang, Ninglian
    Li, Yang
    Li, Xiaofei
    Dong, Zhiwen
    Chen, Pengfei
    SCIENCE OF THE TOTAL ENVIRONMENT, 2017, 574 : 991 - 999
  • [9] Distributions of Polycyclic Aromatic Hydrocarbons, Aromatic Ketones, Carboxylic Acids, and Trace Metals in Arctic Aerosols: Long-Range Atmospheric Transport, Photochemical Degradation/Production at Polar Sunrise
    Singh, Dharmendra Kumar
    Kawamura, Kimitaka
    Yanase, Ayako
    Barrie, Leonard A.
    ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2017, 51 (16) : 8992 - 9004
  • [10] The emerging source of polycyclic aromatic hydrocarbons from mining in the Tibetan Plateau: Distributions and contributions in background soils
    Li, Jun.
    Yuan, Guo-Li
    Li, Ping
    Sun, Yong
    Yu, Hong-Hui
    Wang, Gen-Hou
    SCIENCE OF THE TOTAL ENVIRONMENT, 2017, 584 : 64 - 71