共 102 条
The Technology Horizon for Photocatalytic Water Treatment: Sunrise or Sunset?
被引:579
作者:
Loeb, Stephanie K.
[1
,2
,3
]
Alvarez, Pedro J. J.
[1
,4
]
Brame, Jonathon A.
[5
]
Cates, Ezra L.
[6
]
Choi, Wonyong
[7
]
Crittenden, John
[8
]
Dionysiou, Dionysios D.
[9
]
Li, Qilin
[1
,4
]
Li-Puma, Gianluca
[10
]
Quan, Xie
[11
]
Sedlak, David L.
[12
,13
]
Waite, T. David
[14
]
Westerhoff, Paul
[1
,15
]
Kim, Jae-Hong
[1
,2
,3
]
机构:
[1] Nanosyst Engn Res Ctr Nanotechnol Enabled Water T, 6100 Main St,MS 6398, Houston, TX 77005 USA
[2] Dept Chem & Environm Engn, 17 Hillhouse Ave, New Haven, CT 06511 USA
[3] Yale Univ, 17 Hillhouse Ave, New Haven, CT 06511 USA
[4] Rice Univ, Dept Civil & Environm Engn, 6100 Main St, Houston, TX 77005 USA
[5] US Army, ERDC, 3909 Halls Ferry Rd, Vicksburg, MS 39180 USA
[6] Clemson Univ, Dept Environm Engn & Earth Sci, 342 Comp Court, Anderson, SC 29625 USA
[7] Pohang Univ Sci & Technol, Div Environm Sci & Engn, Pohang 37673, South Korea
[8] Georgia Inst Technol, Sch Civil & Environm Engn, Brook Byers Inst Sustainable Syst, Atlanta, GA 30332 USA
[9] Univ Cincinnati, Dept Chem & Environm Engn, Environm Engn & Sci Program, 705 Engn Res Ctr, Cincinnati, OH 45221 USA
[10] Loughborough Univ, Dept Chem Engn, Environm Nanocatalysis & Photoreact Engn, Loughborough LE11 3TU, Leics, England
[11] Dalian Univ Technol, Sch Environm Sci & Technol, Key Lab Ind Ecol & Environm Engn, Minist Educ, Dalian 116024, Peoples R China
[12] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA
[13] Univ Calif Berkeley, Engn Res Ctr Reinventing Nations Urban Water Infr, Berkeley, CA 94720 USA
[14] Univ New South Wales, Sch Civil & Environm Engn, Sydney, NSW 2052, Australia
[15] Arizona State Univ, Sch Sustainable Engn & Built Environm, Box 3005, Tempe, AZ 85287 USA
关键词:
LIGHT-EMITTING-DIODES;
TITANIUM-DIOXIDE PHOTOCATALYSTS;
ADVANCED OXIDATION PROCESSES;
SOLAR PHOTOCATALYSIS;
WASTE-WATER;
TIO2;
PHOTOCATALYSIS;
QUANTUM YIELDS;
ORGANIC CONTAMINANTS;
HYDROXYL RADICALS;
OH RADICALS;
D O I:
10.1021/acs.est.8b05041
中图分类号:
X [环境科学、安全科学];
学科分类号:
08 ;
0830 ;
摘要:
Advanced oxidation processes via semiconductor photocatalysis for water treatment have been the subject of extensive research over the past three decades, producing many scientific reports focused on elucidating mechanisms and enhancing kinetics for the treatment of contaminants in water. Many of these reports imply that the ultimate goal of the research is to apply photocatalysis in municipal water treatment operations. However, this ignores immense technology transfer problems, perpetuating a widening gap between academic advocation and industrial application. In this Feature, we undertake a critical examination of the trajectory of photocatalytic water treatment research, assessing the viability of proposed applications and identifying those with the most promising future. Several strategies are proposed for scientists and engineers who aim to support research efforts to bring industrially relevant photocatalytic water treatment processes to fruition. Although the reassessed potential may not live up to initial academic hype, an unfavorable assessment in some areas does not preclude the transfer of photocatalysis for water treatment to other niche applications as the technology retains substantive and unique benefits.
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页码:2937 / 2947
页数:11
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