A Two-Step Solution-Processed Wide-Bandgap Perovskite for Monolithic Silicon-Based Tandem Solar Cells with >27% Efficiency

被引：35
作者：
Chen, Bingbing [1 ,2 ,3 ,4 ,5 ]
Wang, Pengyang [1 ,2 ,3 ,4 ,5 ]
Li, Renjie [1 ,2 ,3 ,4 ,5 ]
Ren, Ningyu [1 ,2 ,3 ,4 ,5 ]
Han, Wei [1 ,2 ,3 ,4 ,5 ]
Zhu, Zhao [1 ,2 ,3 ,4 ,5 ]
Wang, Jin [1 ,2 ,3 ,4 ,5 ]
Wang, Sanlong [1 ,2 ,3 ,4 ,5 ]
Shi, Biao [1 ,2 ,3 ,4 ,5 ]
Liu, Jingjing [1 ,2 ,3 ,4 ,5 ]
Liu, Pengfei [1 ,2 ,3 ,4 ,5 ]
Huang, Qian [1 ,2 ,3 ,4 ,5 ]
Xu, Shengzhi [1 ,2 ,3 ,4 ,5 ]
Zhao, Ying [1 ,2 ,3 ,4 ,5 ]
Zhang, Xiaodan [1 ,2 ,3 ,4 ,5 ]
机构：
[1] Nankai Univ, Inst Photoelect Thin Film Devices & Technol, Renewable Energy Convers & Storage Ctr, Solar Energy Res Ctr, Tianjin 300350, Peoples R China
[2] Key Lab Photoelect Thin Film Devices & Technol Tia, Tianjin 300350, Peoples R China
[3] Haihe Lab Sustainable Chem Transformat, Tianjin 300192, Peoples R China
[4] Minist Educ, Engn Res Ctr Thin Film Photoelect Technol, Tianjin 300350, Peoples R China
[5] Collaborat Innovat Ctr Chem Sci & Engn Tianjin, Tianjin 300072, Peoples R China
来源：
ACS ENERGY LETTERS | 2022年 / 7卷 / 08期
基金：
中国国家自然科学基金; 中国博士后科学基金;
关键词：
HALIDE PEROVSKITES;
D O I：
10.1021/acsenergylett.2c01488
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
A two-step solution sequential deposition has been successfully applied to narrow-bandgap (below 1.60 eV) perovskite solar cells (PSCs), while it has not been widely used in wide-bandgap PSCs and monolithic tandem solar cells (TSCs). Here, a lead halide complex is formed by introducing a formamidinium iodide (FAI) and rubidium acetate (RbAc) into the first step. The results show that the lead halide complex alters the crystallization kinetics and promotes a prominent orientation (100) growth of the perovskite film, resulting in an efficiency of 27.64% for monolithic perovskite/silicon TSCs. Additionally, an enlarged-scaled tandem device with an efficiency of 22.81% (active area of 11.879 cm(2)) is also achieved, which is one of the most efficient devices with an area greater than 10 cm(2). This work provides an effective strategy to fabricate perovskite/silicon TSCs with high performance, reproducibility, and large area via the two-step solution method, which will accelerate the industrialization of perovskite/silicon tandem technique.
引用
收藏
页码：2771 / 2780
页数：10
相关论文
共 34 条
[1]   Maximizing and stabilizing luminescence from halide perovskites with potassium passivation [J].
Abdi-Jalebi, Mojtaba ;
Andaji-Garmaroudi, Zahra ;
Cacovich, Stefania ;
Stavrakas, Camille ;
Philippe, Bertrand ;
Richter, Johannes M. ;
Alsari, Mejd ;
Booker, Edward P. ;
Hutter, Eline M. ;
Pearson, Andrew J. ;
Lilliu, Samuele ;
Savenije, Tom J. ;
Rensmo, Hakan ;
Divitini, Giorgio ;
Ducati, Caterina ;
Friend, Richard H. ;
Stranks, Samuel D. .
NATURE, 2018, 555 (7697) :497-+
[2]   A combined molecular dynamics and experimental study of two-step process enabling low-temperature formation of phase-pure α-FAPbI3 [J].
Ahlawat, Paramvir ;
Hinderhofer, Alexander ;
Alharbi, Essa A. ;
Lu, Haizhou ;
Ummadisingu, Amita ;
Niu, Haiyang ;
Invernizzi, Michele ;
Zakeeruddin, Shaik Mohammed ;
Dar, M. Ibrahim ;
Schreiber, Frank ;
Hagfeldt, Anders ;
Graetzel, Michael ;
Rothlisberger, Ursula ;
Parrinello, Michele .
SCIENCE ADVANCES, 2021, 7 (17)
[3]   Monolithic perovskite/silicon tandem solar cell with >29% efficiency by enhanced hole extraction [J].
Al-Ashouri, Amran ;
Kohnen, Eike ;
Li, Bor ;
Magomedov, Artiom ;
Hempel, Hannes ;
Caprioglio, Pietro ;
Marquez, Jose A. ;
Vilches, Anna Belen Morales ;
Kasparavicius, Ernestas ;
Smith, Joel A. ;
Phung, Nga ;
Menzel, Dorothee ;
Grischek, Max ;
Kegelmann, Lukas ;
Skroblin, Dieter ;
Gollwitzer, Christian ;
Malinauskas, Tadas ;
Jost, Marko ;
Matic, Gasper ;
Rech, Bernd ;
Schlatmann, Rutger ;
Topic, Marko ;
Korte, Lars ;
Abate, Antonio ;
Stannowski, Bernd ;
Neher, Dieter ;
Stolterfoht, Martin ;
Unold, Thomas ;
Getautis, Vytautas ;
Albrecht, Steve .
SCIENCE, 2020, 370 (6522) :1300-+
[4]   Insights into the Development of Monolithic Perovskite/Silicon Tandem Solar Cells [J].
Chen, Bingbing ;
Ren, Ningyu ;
Li, Yucheng ;
Yan, Lingling ;
Mazumdar, Sayantan ;
Zhao, Ying ;
Zhang, Xiaodan .
ADVANCED ENERGY MATERIALS, 2022, 12 (04)
[5]   Grain Engineering for Perovskite/Silicon Monolithic Tandem Solar Cells with Efficiency of 25.4% [J].
Chen, Bo ;
Yu, Zhengshan ;
Liu, Kong ;
Zheng, Xiaopeng ;
Liu, Ye ;
Shi, Jianwei ;
Spronk, Derrek ;
Rudd, Peter N. ;
Holman, Zachary ;
Huang, Jinsong .
JOULE, 2019, 3 (01) :177-190
[6]   Mechanical Reliability of Fullerene/Tin Oxide Interfaces in Monolithic Perovskite/Silicon Tandem Cells [J].
De Bastiani, Michele ;
Armaroli, Giovanni ;
Jalmood, Rawan ;
Ferlauto, Laura ;
Li, Xiaole ;
Tao, Ran ;
Harrison, George T. ;
Eswaran, Mathan K. ;
Azmi, Randi ;
Babics, Maxime ;
Subbiah, Anand S. ;
Aydin, Erkan ;
Allen, Thomas G. ;
Combe, Craig ;
Cramer, Tobias ;
Baran, Derya ;
Schwingenschlogl, Udo ;
Lubineau, Gilles ;
Cavalcoli, Daniela ;
De Wolf, Stefaan .
ACS ENERGY LETTERS, 2022, 7 (02) :827-833
[7]   Photo-induced halide redistribution in organic-inorganic perovskite films [J].
deQuilettes, Dane W. ;
Zhang, Wei ;
Burlakov, Victor M. ;
Graham, Daniel J. ;
Leijtens, Tomas ;
Osherov, Anna ;
Bulovic, Vladimir ;
Snaith, Henry J. ;
Ginger, David S. ;
Stranks, Samuel D. .
NATURE COMMUNICATIONS, 2016, 7
[8]   Ionic transport in hybrid lead iodide perovskite solar cells [J].
Eames, Christopher ;
Frost, Jarvist M. ;
Barnes, Piers R. F. ;
O'Regan, Brian C. ;
Walsh, Aron ;
Islam, M. Saiful .
NATURE COMMUNICATIONS, 2015, 6
[9]   Monolithic Perovskite-Silicon Tandem Solar Cells: From the Lab to Fab? [J].
Fu, Fan ;
Li, Jia ;
Yang, Terry Chien-Jen ;
Liang, Haoming ;
Faes, Antonin ;
Jeangros, Quentin ;
Ballif, Christophe ;
Hou, Yi .
ADVANCED MATERIALS, 2022, 34 (24)
[10]   Control Perovskite Crystals Vertical Growth for Obtaining High-Performance Monolithic Perovskite/Silicon Heterojunction Tandem Solar Cells with VOC of 1.93 V [J].
Hou, Fuhua ;
Li, Yucheng ;
Yan, Lingling ;
Shi, Biao ;
Ren, Ningyu ;
Wang, Pengyang ;
Zhang, Dekun ;
Ren, Huizhi ;
Ding, Yi ;
Huang, Qian ;
Li, Tiantian ;
Li, Yuelong ;
Zhao, Ying ;
Zhang, Xiaodan .
SOLAR RRL, 2021, 5 (10)
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