Integrated Modeling of US Agricultural Soil Emissions of Reactive Nitrogen and Associated Impacts on Air Pollution, Health, and Climate

被引:19
作者
Luo, Lina [1 ]
Ran, Limei [2 ]
Rasool, Quazi Z. [3 ]
Cohan, Daniel S. [1 ]
机构
[1] Rice Univ, Dept Civil & Environm Engn, Houston, TX 77005 USA
[2] USDA, Nat Resources Conservat Serv, Greensboro, NC 27401 USA
[3] Pacific Northwest Natl Lab, Richland, WA 99352 USA
关键词
agricultural soil emissions; nitrogen oxides (NOx); ammonia (NH3); nitrous oxide (N2O); agroecosystem models; FEST-C; reduced-form air quality and health models; APEEP; FINE-PARTICULATE MATTER; OXIDE EMISSIONS; SENSITIVITY-ANALYSIS; N2O EMISSIONS; SOURCE APPORTIONMENT; PRECURSOR EMISSIONS; NONLINEAR RESPONSE; AMMONIA EMISSIONS; INORGANIC PM2.5; USE EFFICIENCY;
D O I
10.1021/acs.est.1c08660
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Agricultural soils are leading sources of reactive nitrogen (Nr) species including nitrogen oxides (NOx), ammonia (NH3), and nitrous oxide (N2O). The propensity of NOx and NH3 to generate ozone and fine particulate matter and associated impacts on health are highly variable, whereas the climate impacts of long-lived N2O are independent of emission timing and location. However, these impacts have rarely been compared on a spatially resolved monetized basis. In this study, we update the nitrogen scheme in an agroecosystem model to simulate the Nr emissions from fertilized soils across the contiguous United States. We then apply a reduced-form air pollution health effect model to assess air quality impacts from NOx and NH3 and a social cost of N2O to assess the climate impacts. Assuming an $8.2 million value of a statistical life and a $13,100/ton social cost of N2O, the air quality impacts are a factor of similar to 7 to 15 times as large as the climate impacts in heavily populated coastal regions, whereas the ratios are closer to 2.5 in sparsely populated regions. Our results show that air pollution, health, and climate should be considered jointly in future assessments of how farming practices affect Nr emissions.
引用
收藏
页码:9265 / 9276
页数:12
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