Carbon dioxide uptake from natural gas by binary ionic liquid-water mixtures

被引：71

作者：

Anderson, Kris ^{[1
]}

Atkins, Martin P. ^{[1
]}

Estager, Julien ^{[1
]}

Kuah, Yongcheun ^{[1
]}

Ng, Shieling ^{[1
]}

Oliferenko, Alexander A. ^{[1
]}

Plechkova, Natalia V. ^{[1
]}

Puga, Alberto V. ^{[1
]}

Seddon, Kenneth R. ^{[1
]}

Wassell, David F. ^{[1
]}

机构：

[1] Queens Univ Belfast, Sch Chem & Chem Engn, QUILL Res Ctr, Belfast BT9 5AG, Antrim, North Ireland

来源：

GREEN CHEMISTRY | 2015年 / 17卷 / 08期

关键词：

RAMAN-SPECTROSCOPY; PHASE-BEHAVIOR; CO2; CAPTURE; ABSORPTION; ACETATE; SOLUBILITY; CHEMISORPTION; TEMPERATURE; PLUS;

D O I：

10.1039/c5gc00720h

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Carbon dioxide solubility in a set of carboxylate ionic liquids formulated with stoicheiometric amounts of water is found to be significantly higher than for other ionic liquids previously reported. This is due to synergistic chemical and physical absorption. The formulated ionic liquid/water mixtures show greatly enhanced carbon dioxide solubility relative to both anhydrous ionic liquids and aqueous ionic liquid solutions, and are competitive with commercial chemical absorbers, such as activated N-methyldiethanolamine or monoethanolamine.

引用

收藏

页码：4340 / 4354

页数：15

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