A Visible-Light-Driven Z-Scheme CO2 Reduction System Using Ta3N5 and a Ru(II) Binuclear Complex

被引：26

作者：

Muraoka, Kanemichi ^{[1
,2
]}

Uchiyama, Tomoki ^{[3
]}

Lu, Daling ^{[4
]}

Uchimoto, Yoshiharu ^{[3
]}

Ishitani, Osamu ^{[1
]}

Maeda, Kazuhiko ^{[1
]}

机构：

[1] Tokyo Inst Technol, Sch Sci, Dept Chem, Meguro Ku, Tokyo 1528550, Japan

[2] Japan Soc Promot Sci, Chiyoda Ku, Kojimachi Business Ctr Bldg 5-3-1, Tokyo 1020083, Japan

[3] Kyoto Univ, Grad Sch Human & Environm Studies, Sakyo Ku, Yoshida Nihonmatsu Cho, Kyoto 6068501, Japan

[4] Tokyo Inst Technol, Tech Dept, Suzukakedai Mat Anal Div, Midori Ku, 4259 Nagatsuta Cho, Yokohama, Kanagawa 2268503, Japan

来源：

BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN | 2019年 / 92卷 / 01期

关键词：

Artificial photosynthesis; Heterogeneous photocatalysis; Solar fuels; GRAPHITIC CARBON NITRIDE; METAL-COMPLEX; PHOTOCATALYTIC REDUCTION; TANTALUM OXYNITRIDE; WATER; SEMICONDUCTOR; HYBRID; CONVERSION; TA2O5;

D O I：

10.1246/bcsj.20180239

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

A hybrid photocatalyst constructed with Ta3N5 and a binuclear ruthenium(II) complex had the ability to reduce CO2 into formate with >99% selectivity under visible light (lambda > 480 nm), presenting the first report of a semiconductor material with a 600-nm absorption edge that is operable in a metal-complex/semiconductor photocatalyst.

引用

页码：124 / 126

页数：3

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