A Visible-Light-Driven Z-Scheme CO2 Reduction System Using Ta3N5 and a Ru(II) Binuclear Complex

被引：25
|
作者：
Muraoka, Kanemichi [1 ,2 ]
Uchiyama, Tomoki [3 ]
Lu, Daling [4 ]
Uchimoto, Yoshiharu [3 ]
Ishitani, Osamu [1 ]
Maeda, Kazuhiko [1 ]
机构：
[1] Tokyo Inst Technol, Sch Sci, Dept Chem, Meguro Ku, Tokyo 1528550, Japan
[2] Japan Soc Promot Sci, Chiyoda Ku, Kojimachi Business Ctr Bldg 5-3-1, Tokyo 1020083, Japan
[3] Kyoto Univ, Grad Sch Human & Environm Studies, Sakyo Ku, Yoshida Nihonmatsu Cho, Kyoto 6068501, Japan
[4] Tokyo Inst Technol, Tech Dept, Suzukakedai Mat Anal Div, Midori Ku, 4259 Nagatsuta Cho, Yokohama, Kanagawa 2268503, Japan
来源：
BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN | 2019年 / 92卷 / 01期
关键词：
Artificial photosynthesis; Heterogeneous photocatalysis; Solar fuels; GRAPHITIC CARBON NITRIDE; METAL-COMPLEX; PHOTOCATALYTIC REDUCTION; TANTALUM OXYNITRIDE; WATER; SEMICONDUCTOR; HYBRID; CONVERSION; TA2O5;
D O I：
10.1246/bcsj.20180239
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
A hybrid photocatalyst constructed with Ta3N5 and a binuclear ruthenium(II) complex had the ability to reduce CO2 into formate with >99% selectivity under visible light (lambda > 480 nm), presenting the first report of a semiconductor material with a 600-nm absorption edge that is operable in a metal-complex/semiconductor photocatalyst.
引用
收藏
页码：124 / 126
页数：3
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