High-order harmonic generation from hybrid organic-inorganic perovskite thin films

被引：45

作者：

Hirori, Hideki ^{[1
]}

Xia, Peiyu ^{[2
]}

Shinohara, Yasushi ^{[3
,4
]}

Otobe, Tomohito ^{[5
]}

Sanari, Yasuyuki ^{[1
]}

Tahara, Hirokazu ^{[1
]}

Ishii, Nobuhisa ^{[2
]}

Itatani, Jiro ^{[2
]}

Ishikawa, Kenichi L. ^{[3
,4
,6
]}

Aharen, Tomoko ^{[1
]}

Ozaki, Masashi ^{[1
]}

Wakamiya, Atsushi ^{[1
]}

Kanemitsu, Yoshihiko ^{[1
]}

机构：

[1] Kyoto Univ, Inst Chem Res, Uji, Kyoto 6110011, Japan

[2] Univ Tokyo, Inst Solid State Phys, Kashiwa, Chiba 2778581, Japan

[3] Univ Tokyo, Photon Sci Ctr, Grad Sch Engn, Bunkyo Ku, Tokyo 1138656, Japan

[4] Univ Tokyo, Grad Sch Engn, Dept Nucl Engn & Management, Bunkyo Ku, Tokyo 1138656, Japan

[5] Natl Inst Quantum & Radiol Sci & Technol, Kansai Photon Sci Inst, Kyoto 6190615, Japan

[6] Univ Tokyo, Res Inst Photon Sci & Laser Technol, Bunkyo Ku, Tokyo 1130033, Japan

来源：

APL MATERIALS | 2019年 / 7卷 / 04期

关键词：

HALIDE PEROVSKITES;

D O I：

10.1063/1.5090935

中图分类号：

TB3 [工程材料学];

学科分类号：

0805 ; 080502 ;

摘要：

The generation of high-order harmonics from hybrid organic-inorganic perovskites (HOIPs) is demonstrated by the excitation with a strong mid-infrared laser pulse. We prepare three types of HOIP polycrystalline thin film samples by solution processes (MAPbX(3); MA = CH3NH3+; X = I, Br, Cl). The high-order harmonics from the sample (MAPbBr(3)) are more than tenfold stronger than those from the well-studied GaSe crystal despite their comparable bandgap energies, implying that the stronger band-to-band transition of the HOIPs causes the higher yields. (C) 2019 Author(s).

引用

页数：4

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