Directional Emission from Electrically Injected Exciton-Polaritons in Perovskite Metasurfaces

被引:13
作者
Wang, Yutao [1 ,2 ,3 ]
Tian, Jingyi [1 ,2 ]
Klein, Maciej [1 ,2 ]
Adamo, Giorgio [1 ,2 ]
Ha, Son Tung [4 ]
Soci, Cesare [1 ,2 ]
机构
[1] Nanyang Technol Univ, Ctr Disrupt Photon Technol, Sch Phys & Math Sci, TPI, Singapore 637371, Singapore
[2] Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore
[3] Nanyang Technol Univ, Energy Res Inst NTU ERI N, Interdisciplinary Grad Sch, Singapore 637553, Singapore
[4] ASTAR, Inst Mat Res & Engn, Singapore 138634, Singapore
关键词
metal halide perovskites; electrically injected exciton-polaritons; dielectric metasurfaces; bound states in the continuum; light-emitting transistor; strong coupling;
D O I
10.1021/acs.nanolett.3c00727
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We present a new approach to achieving strong coupling between electrically injected excitons and photonic bound states in the continuum of a dielectric metasurface. Here a high-finesse metasurface cavity is monolithically patterned in the channel of a perovskite light-emitting transistor to induce a large Rabi splitting of similar to 200 meV and more than 50-fold enhancement of the polaritonic emission compared to the intrinsic excitonic emission of the perovskite film. Moreover, the directionality of polaritonic electroluminescence can be dynamically tuned by varying the source-drain bias, which induces an asymmetric distribution of exciton population within the transistor channel. We argue that this approach provides a new platform to study strong light-matter interactions in dispersion engineered photonic cavities under electrical injection and paves the way to solution-processed electrically pumped polariton lasers.
引用
收藏
页码:4431 / 4438
页数:8
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