Effects of mechanically-induced oscillations on soot formation and flame temperature in laminar diffusion flames of ethylene

An experimental study was performed to measure the effects of flame oscillations on soot concentration and flame temperature in co-flow laminar diffusion flames of ethylene. One novel aspect of this study is that flame oscillations were mechanically induced by moving the burner assembly in a reciprocating motion with an industrial computer-controlled linear stage. Motor speed was used to control the oscillation frequency. The peak-to-peak oscillation amplitude was defined as stroke, which was then used to calculate the Strouhal number. Oscillation frequencies of 5-20 Hz and peak-to-peak amplitudes of 0.5-3 mm were studied. At 1 mm peak-to-peak oscillation amplitude, flame oscillations switched from tip flickering type to tip-clipping type oscillations above 10 Hz. Time-averaged soot concentration increased from its value in the steady-state flame when the flame was perturbed by small oscillation frequencies and amplitudes but then decreased as the oscil-lation intensity was increased. The peak time-averaged soot volume fraction was 9.5 ppm in the steady-state flame and 4.5 ppm at a peak-to-peak oscillation amplitude and an oscillation frequency of 1 mm and 20 Hz, respectively. Similarly, the peak soot volume fraction was 5.8 ppm at a peak-to-peak oscillation amplitude and an oscillation frequency of 3 mm and 10 Hz, respectively. The time-averaged flame temperatures were in the range of 1500-2000 K. The low-temperature zone was observed at the flame core in the steady-state flame and for low-intensity oscillations, and at the flame tip for high-intensity oscillations. The literature has discrepancies on how flame oscillations affect the total soot loading in ethylene flames. Our results show that the total soot loading increased by about 10% from steady-state to low-intensity oscillations, then slightly decreased as either oscillation frequency or amplitude was increased. The effects of increasing the oscillation frequency or amplitude were similar and well captured by the revised Strouhal number. Crown Copyright & COPY; 2022 Published by Elsevier Inc. on behalf of The Combustion Institute. All rights reserved.