The Preparation of Mn-Modified CeO2 Nanosphere Catalysts and Their Catalytic Performance for Soot Combustion

被引:8
作者
Gao, Siyu [1 ]
Yu, Di [2 ]
Zhou, Shengran [1 ]
Zhang, Chunlei [1 ]
Wang, Lanyi [2 ]
Fan, Xiaoqiang [1 ]
Yu, Xuehua [1 ]
Zhao, Zhen [1 ,2 ]
机构
[1] Shenyang Normal Univ, Inst Catalysis Energy & Environm, Coll Chem & Chem Engn, 253 Huanghe North St, Shenyang 110034, Peoples R China
[2] China Univ Petr, State Key Lab Heavy Oil Proc, 18 Fuxue Rd, Beijing 102249, Peoples R China
关键词
MnOx/CeO2; nanospheres; soot combustion; catalysts; MIXED OXIDES; MANGANESE OXIDE; SOLID-SOLUTIONS; NANOROD-LIKE; OXYGEN; OXIDATION; COMPOSITES; RESISTANCE; MORPHOLOGY; REDUCTION;
D O I
10.3390/pr11102902
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
With the increasing stringency of environmental protection regulations, reducing the severe pollution caused by soot particles from diesel vehicle exhaust has become a widespread concern. Catalytic purification technology is currently an efficient method for eliminating soot particles, which needs to develop high-activity catalysts. This work uses a two-step hydrothermal method to synthesize MnOx/CeO2 nanosphere catalysts, which have synergistic effects between manganese and cerium, and have high reactive oxygen species. Among them, the MnCe-1:4 catalyst represents the optimal catalytic activity, and the values of T-10, T-50, and T-90 are 289, 340, and 373 degrees C, respectively. On account of their simple synthetic procedure and low cost, the prepared MnOx/CeO2 nanosphere catalysts have good prospects for practical applications.
引用
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页数:14
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