The self-assembly of a pair of low-symmetry tetracarboxylic acid molecules and their co-assembly with bridging molecules at the liquid-solid interface

被引：11
|
作者：
Zhang, Siqi [1 ,2 ]
Li, Jianqiao [2 ]
Gan, Linlin [2 ]
Ma, Lin [2 ]
Ma, Wei [4 ]
Zhang, Min [1 ]
Cheng, Faliang [1 ]
Deng, Ke [2 ]
Zeng, Qingdao [2 ,3 ]
机构：
[1] Dongguan Univ Technol, Guangdong Engn & Technol Res Ctr Adv Nanomat, Sch Environm & Civil Engn, Dongguan 523808, Peoples R China
[2] Natl Ctr Nanosci & Technol NCNST, CAS Ctr Excellence Nanosci, CAS Key Lab Standardizat & Measurement Nanotechnol, Beijing 100190, Peoples R China
[3] Univ Chinese Acad Sci, Ctr Mat Sci & Optoelect Engn, Beijing 100049, Peoples R China
[4] Xi An Jiao Tong Univ, State Key Lab Mech Behav Mat, Xian 710049, Peoples R China
来源：
NANOSCALE | 2023年 / 15卷 / 09期
基金：
中国国家自然科学基金;
关键词：
SUPRAMOLECULAR ASSEMBLIES; DERIVATIVES; NETWORKS; RECOGNITION; DEPOSITION;
D O I：
10.1039/d2nr06740d
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
The supramolecular self-assembly behavior of a pair of low-symmetry tetracarboxylic acid molecules (H4OBDB and H(4)ADDI) and their co-assembly behavior with TMA as a bridging molecule were studied at the liquid-solid interface. Scanning tunneling microscope (STM) observations revealed that H4OBDB and H(4)ADDI molecules both tend to form O-shaped dimers but end up forming different types of self-assembly structures. We also investigated the construction of two-component co-assembly structures by mixing H4OBDB or H(4)ADDI molecules with bridging molecules such as TMA. The two formed co-assembly structures are similar. Based on the analysis of the STM results and the density functional theory (DFT) calculations, the formation mechanism of the assembled structures was revealed.
引用
收藏
页码：4353 / 4360
页数：8
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