Solar driven photocatalytic disinfection by Z-scheme heterojunction of In2O3/g-C3N4: Performance, mechanism and application

被引:49
作者
Chen, Xiongjian [1 ]
Jin, Yanchao [1 ,5 ]
Huang, Peiwen [1 ]
Zheng, Zhanwang [2 ]
Li, Li-Ping [3 ]
Lin, Chun-Yan [4 ]
Chen, Xiao [1 ,5 ]
Ding, Rui [1 ,5 ]
Liu, Jianxi [1 ,5 ]
Chen, Riyao [1 ,5 ]
机构
[1] Fujian Normal Univ, Coll Environm & Resource Sci, Fuzhou 350117, Fujian, Peoples R China
[2] Zhejiang Sunda Publ Environm Protect Co Ltd, Hangzhou 310012, Peoples R China
[3] Beijing Normal Univ, Res & Dev Ctr Watershed Environm Ecoengn, Zhuhai 519087, Peoples R China
[4] Minjiang Univ, Sch Mat & Chem Engn, Fuzhou 350108, Fujian, Peoples R China
[5] Fujian Key Lab Pollut Control & Resource Reuse, Fuzhou 350117, Peoples R China
来源
APPLIED CATALYSIS B-ENVIRONMENT AND ENERGY | 2024年 / 340卷
基金
中国国家自然科学基金;
关键词
Photocatalytic disinfection; G-C3N4; Indium oxide; Z-scheme heterojunction; BACTERIAL INACTIVATION; G-C3N4; COMPOSITE; WATER; NANOCOMPOSITES; ENHANCEMENT; ACTIVATION; OXIDATION; ACID; AG;
D O I
10.1016/j.apcatb.2023.123235
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
To realize an efficient solar disinfection, Z-scheme In2O3/g-C3N4 heterojunctions were prepared and its performances were investigated. The In2O3/g-C3N4 exhibits a wide light response range and a low carrier recombination rate. Due to the transfer of electron (e(-)) and hole (h(+)) between In2O3 and g-C3N4, the generations of superoxide (O-2(center dot-)) and hydroxyl radicals (HO center dot) were enhanced. O2 center dot - HO center dot and h(+) played important roles for disinfection. Approximately 10(6) CFU/mL E. coli were inactivated within 90 min. In addition to cell membrane lysis, DNA was degraded. In2O3/g-C3N4 still revealed high sterilization efficiencies under natural sunlight or for actual wastewater treatment. Although humic acid and inorganic anions (Cl- < NO3- < SO42- < H2PO4- < HCO3-) inhibited the disinfection, detection limit (DL, about 5.8-log removal) can be achieved. Furthermore, DL still could be achieved and the In2O3/g-C3N4 structure remained intact after 5 cycles. This study provides novel guidance for solar-driven water purification.
引用
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页数:12
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