Experimental study and optimization of flow field structures in proton exchange membrane fuel cell under different anode modes

被引:5
作者
Meng, Xiangchao [1 ,2 ]
Ren, Hong [1 ,2 ]
Xie, Feng [1 ]
Shao, Zhigang [1 ]
机构
[1] Chinese Acad Sci, Dalian Inst Chem Phys, Fuel Cell Syst & Engn Lab, Key Lab Fuel Cells Hybrid Power Sources,, Dalian 116023, Peoples R China
[2] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
关键词
Flow field structure; Water management; Anode modes; Current density distribution; Pressure drop; IMPEDANCE SPECTROSCOPY; WATER REMOVAL; PERFORMANCE; DESIGN; TRANSPORT; GEOMETRY; PARALLEL; TEMPERATURE; PARAMETERS; MANAGEMENT;
D O I
10.1016/j.ijhydene.2023.03.229
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
As one of the critical components in the proton exchange membrane fuel cell (PEMFC), the flow field is crucial to the improvement of cell performance. However, the current research on flow field structure lacks consideration of the influence of different anode modes, which makes the existing flow field structure rules have limitations in the practical application of PEMFC. In this paper, the PEMFC characteristics of parallel flow field, S-shaped flow field, multi-serpentine flow field and single-serpentine flow field at the cathode side are compared experimentally in the dead-end anode (DEA) mode and hydrogen circulation anode (HCA) mode, respectively. Especially, the spatial current density distribution and parasitic power of different flow field structures are measured. The results show that the performance trends of different flow field structures change with the DEA and HCA anode modes. In DEA mode, the PEMFC is prone to flooding, and the flow field with high gas velocity in the channel has better drainage ability, which can obtain higher cell perfor-mance. The HCA mode is helpful for the discharge of water in the PEMFC, which effectively alleviates the adverse impact of water accumulation on the overall performance, and the mass transport ability of the flow field structure plays a leading role in the cell performance improvement. In addition, although the high gas flow velocity has better drainage ability in the flow field, it may lead to a decrease in the current density distribution uniformity and PEMFC net output power density. Based on the comprehensive consideration of the experimental results, the multi-serpentine flow field is more suitable for DEA mode, and the S-shaped flow field is more suitable for HCA mode.& COPY; 2023 Published by Elsevier Ltd on behalf of Hydrogen Energy Publications LLC.
引用
收藏
页码:24447 / 24458
页数:12
相关论文
共 46 条
[1]   Simultaneous direct visualisation of liquid water in the cathode and anode serpentine flow channels of proton exchange membrane (PEM) fuel cells [J].
Aslam, R. M. ;
Ingham, D. B. ;
Ismail, M. S. ;
Hughes, K. J. ;
Ma, L. ;
Pourkashanian, M. .
JOURNAL OF THE ENERGY INSTITUTE, 2018, 91 (06) :1057-1070
[2]   Topology optimization as a powerful tool to design advanced PEMFCs flow fields [J].
Behrou, Reza ;
Pizzolato, Alberto ;
Forner-Cuenca, Antoni .
INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER, 2019, 135 :72-92
[3]   Operation characteristics and carbon corrosion of PEMFC (Proton exchange membrane fuel cell) with dead-ended anode for high hydrogen utilization [J].
Chen, Ben ;
Ke, Wandi ;
Luo, Maji ;
Wang, Jun ;
Tu, Zhengkai ;
Pan, Mu ;
Zhang, Haining ;
Liu, Xiaowei ;
Liu, Wei .
ENERGY, 2015, 91 :799-806
[4]   Transport phenomena of convergent and divergent serpentine flow fields for PEMFC [J].
Chowdhury, Mohammad Ziauddin ;
Timurkutluk, Bora .
ENERGY, 2018, 161 :104-117
[5]   Experimental optimization of parallel and interdigitated PEMFC flow-field channel geometry [J].
Cooper, Nathanial J. ;
Smith, Travis ;
Santamaria, Anthony D. ;
Park, Jae Wan .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2016, 41 (02) :1213-1223
[6]   Durability and degradation issues of PEM fuel cell components [J].
de Bruijn, F. A. ;
Dam, V. A. T. ;
Janssen, G. J. M. .
FUEL CELLS, 2008, 8 (01) :3-22
[7]   Experimental study of the S-shaped flow fields in proton exchange membrane fuel cells [J].
He, Liang ;
Hou, Ming ;
Gao, Yanyan ;
Sun, Xinye ;
Song, Wei ;
Zheng, Liming ;
Ai, Jun ;
Zhang, Hongjie ;
Shao, Zhigang .
ENERGY CONVERSION AND MANAGEMENT, 2020, 223
[8]   A novel three-dimensional flow field design and experimental research for proton exchange membrane fuel cells [J].
He, Liang ;
Hou, Ming ;
Gao, Yanyan ;
Fang, Dahui ;
Wang, Penghao ;
Lv, Bo ;
Shao, Zhigang .
ENERGY CONVERSION AND MANAGEMENT, 2020, 205
[9]   Effect of hydrogen delivery schemes on fuel cell efficiency [J].
Hwang, Jenn-Jiang .
JOURNAL OF POWER SOURCES, 2013, 239 :54-63
[10]   Energy efficiency improvements by investigating the water flooding management on proton exchange membrane fuel cell (PEMFC) [J].
Ijaodola, O. S. ;
El-Hassan, Zaki ;
Ogungbemi, E. ;
Khatib, F. N. ;
Wilberforce, Tabbi ;
Thompson, James ;
Olabi, A. G. .
ENERGY, 2019, 179 :246-267