Friction Characteristics of Two-Dimensional Hybrid Organic-Inorganic Perovskites

被引:1
作者
Van, V. K. H. [1 ]
DelRio, F. W. [2 ]
Tu, Q. [3 ]
Chung, K. -H. [1 ]
机构
[1] Univ Ulsan, Sch Mech Engn, 93 Daehak Ro, Ulsan 44610, South Korea
[2] Sandia Natl Labs, Mat Phys & Chem Sci Ctr, Albuquerque, NM 87185 USA
[3] Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77843 USA
基金
新加坡国家研究基金会;
关键词
Friction force microscopy; Perovskites; Thickness dependent friction; Chain length; PHASE-TRANSITIONS; MECHANICAL-PROPERTIES; HYDROGEN-PRODUCTION; (CNH2N+1NH3)(2)PBI4; CALIBRATION; SOLAR;
D O I
10.1007/s11340-023-00967-6
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
BackgroundTwo-dimensional (2D) hybrid organic-inorganic perovskites (HOIPs) have been and continue to be of great interest to researchers, given their use in flexible solar cells, wearable sensors, and electronic devices. Frictional properties of 2D HOIPs should be clearly understood to establish the manufacturing processes as well as the durability of the devices.ObjectiveThe aim of this study is to provide a fundamental understanding of the frictional properties of 2D HOIPs at the nanoscale.MethodsThe topography of 2D HOIPs with three different chain lengths and five different thicknesses were systematically examined with atomic force microscopy (AFM). The frictional properties of these films were also quantitatively assessed under various normal forces using friction force microscopy (FFM).ResultsFrom the AFM, it was found that the 2D HOIPs exhibited nanoscale surface roughness, presumably due to local disorder of the organic cations or deformation of the inorganic framework. In addition, FFM showed that the intrinsic friction of 2D HOIPs was significantly low. The friction force decreased as molecular chain length increased and thickness-dependent friction characteristics were clearly observed.ConclusionsThe trends were due to changes in mechanical properties, surface roughness, and suppression of puckering, but not due to changes in AFM tip adhesion.
引用
收藏
页码:1085 / 1090
页数:6
相关论文
共 37 条
[1]   Layer-dependent anisotropic frictional behavior in two-dimensional monolayer hybrid perovskite/ITO layered heterojunctions [J].
Bi, Sheng ;
Li, Qikun ;
Yan, Ying ;
Asare-Yeboah, Kyeiwaa ;
Ma, Tianbao ;
Tang, Chaolong ;
Ouyang, Zhongliang ;
He, Zhengran ;
Liu, Yun ;
Jiang, Chengming .
PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2019, 21 (05) :2540-2546
[2]   Quantitative assessment of contact and non-contact lateral force calibration methods for atomic force microscopy [J].
Bien Cuong Tran Khac ;
Chung, Koo-Hyun .
ULTRAMICROSCOPY, 2016, 161 :41-50
[3]   Synthesis, characterization and phase transitions in the inorganic-organic layered perovskite-type hybrids [(CnH2n+1NH3)2PbI4], n=4, 5 and 6 [J].
Billing, David G. ;
Lemmerer, Andreas .
ACTA CRYSTALLOGRAPHICA SECTION B-STRUCTURAL SCIENCE CRYSTAL ENGINEERING AND MATERIALS, 2007, 63 (735-747) :735-747
[4]   Synthesis, characterization and phase transitions of the inorganic-organic layered perovskite-type hybrids [(CnH2n+1NH3)2PbI4] (n=12, 14, 16 and 18) [J].
Billing, David G. ;
Lemmerer, Andreas .
NEW JOURNAL OF CHEMISTRY, 2008, 32 (10) :1736-1746
[5]   A review on exergy comparison of hydrogen production methods from renewable energy sources [J].
Christopher, Koroneos ;
Dimitrios, Rovas .
ENERGY & ENVIRONMENTAL SCIENCE, 2012, 5 (05) :6640-6651
[6]   Fundamental Investigation of the Wear Progression of Silicon Atomic Force Microscope Probes [J].
Chung, Koo-Hyun ;
Lee, Yong-Ha ;
Kim, Hae-Jin ;
Kim, Dae-Eun .
TRIBOLOGY LETTERS, 2013, 52 (02) :315-325
[7]   Note: Lateral force microscope calibration using multiple location pivot loading of rectangular cantilevers [J].
Chung, Koo-Hyun ;
Reitsma, Mark G. .
REVIEW OF SCIENTIFIC INSTRUMENTS, 2010, 81 (02)
[8]   Atomically thin two-dimensional organic-inorganic hybrid perovskites [J].
Dou, Letian ;
Wong, Andrew B. ;
Yu, Yi ;
Lai, Minliang ;
Kornienko, Nikolay ;
Eaton, Samuel W. ;
Fu, Anthony ;
Bischak, Connor G. ;
Ma, Jie ;
Ding, Tina ;
Ginsberg, Naomi S. ;
Wang, Lin-Wang ;
Alivisatos, A. Paul ;
Yang, Peidong .
SCIENCE, 2015, 349 (6255) :1518-1521
[9]   Preface: Overview of the forum on solar and renewable energy [J].
Eisenberg, R ;
Nocera, DG .
INORGANIC CHEMISTRY, 2005, 44 (20) :6799-6801
[10]   Thickness dependent friction on few-layer MoS2, WS2, and WSe2 [J].
Fang, Liang ;
Liu, Da-Meng ;
Guo, Yuzheng ;
Liao, Zhi-Min ;
Luo, Jian-Bin ;
Wen, Shi-Zhu .
NANOTECHNOLOGY, 2017, 28 (24)