Tap Reactor for Temporally and Spatially Resolved Analysis of the CO2 Methanation Reaction

被引:1
|
作者
Engl, Timo [1 ]
Langer, Moritz [2 ]
Freund, Hannsjoerg [2 ]
Rubin, Michael [1 ,3 ]
Dittmeyer, Roland [3 ]
机构
[1] Karlsruhe Inst Technol, Inst Micro Proc Engn IMVT, Hermann Von Helmholtz Pl 1, D-76344 Eggenstein Leopoldshafen, Germany
[2] TU Dortmund Univ, Inst React Engn & Catalysis REC, Emil Figge Str 66, D-44227 Dortmund, Germany
[3] Karlsruhe Inst Technol, Inst Catalysis Res & Technol IKFT, Hermann Von Helmholtz Pl 1, D-76344 Eggenstein Leopoldshafen, Germany
关键词
Catalyst coatings; CO2; methanation; Spatially and temporally resolved analysis; Tap reactors; Transient operation; CATALYTIC PARTIAL OXIDATION; PROFILES; KINETICS; STORAGE; IMPACT; RH;
D O I
10.1002/cite.202200204
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Chemical energy carriers produced according to power-to-X concepts will play a crucial role in the future energy system. Here, CO2 methanation is described as one promising route. However, transient operating conditions and the resulting effects on catalyst stability are to be considered. In this contribution, a tap reactor for spatially and temporally resolved analysis of the methanation reaction is presented. The Ni catalyst investigated was implemented as coating. Reaction data as a function of time and reactor coordinate under various operating conditions are presented and discussed. A comparison with simulation data validates the presented tap reactor concept.
引用
收藏
页码:658 / 667
页数:10
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