Principles of Design and Synthesis of Metal Derivatives from MOFs

被引:102
作者
De Villenoisy, Thibault [1 ]
Zheng, Xiaoran [1 ]
Wong, Vienna [1 ]
Mofarah, Sajjad S. [1 ]
Arandiyan, Hamidreza [2 ,3 ]
Yamauchi, Yusuke [4 ]
Koshy, Pramod [1 ]
Sorrell, Charles C. [1 ]
机构
[1] UNSW Sydney, Sch Mat Sci & Engn, Sydney, NSW 2052, Australia
[2] RMIT Univ, Ctr Adv Mat & Ind Chem CAMIC, Melbourne, Vic 3000, Australia
[3] Univ Sydney, Sch Chem, Lab Adv Catalysis Sustainabil, Sydney, NSW 2006, Australia
[4] Univ Queensland, Australian Inst Bioengn & Nanotechnol AIBN, St Lucia, Qld 4072, Australia
关键词
design and synthesis; metal-based derivatives; metal-organic frameworks; MOF-derived materials; N-DOPED CARBON; ORGANIC FRAMEWORKS MOFS; REDUCED GRAPHENE OXIDE; HIGH-PERFORMANCE ANODE; OXYGEN EVOLUTION; HYDROGEN EVOLUTION; ION BATTERY; IN-SITU; BIFUNCTIONAL ELECTROCATALYSTS; ELECTROCHEMICAL DEPOSITION;
D O I
10.1002/adma.202210166
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Materials derived from metal-organic frameworks (MOFs) have demonstrated exceptional structural variety and complexity and can be synthesized using low-cost scalable methods. Although the inherent instability and low electrical conductivity of MOFs are largely responsible for their low uptake for catalysis and energy storage, a superior alternative is MOF-derived metal-based derivatives (MDs) as these can retain the complex nanostructures of MOFs while exhibiting stability and electrical conductivities of several orders of magnitude higher. The present work comprehensively reviews MDs in terms of synthesis and their nanostructural design, including oxides, sulfides, phosphides, nitrides, carbides, transition metals, and other minor species. The focal point of the approach is the identification and rationalization of the design parameters that lead to the generation of optimal compositions, structures, nanostructures, and resultant performance parameters. The aim of this approach is to provide an inclusive platform for the strategies to design and process these materials for specific applications. This work is complemented by detailed figures that both summarize the design and processing approaches that have been reported and indicate potential trajectories for development. The work is also supported by comprehensive and up-to-date tabular coverage of the reported studies.
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页数:53
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