A Decade of Electrocatalysis with Metal Aerogels: A Perspective

被引:19
作者
Li, Weishan [1 ]
Weng, Beibei [1 ]
Sun, Xiaoyue [1 ]
Cai, Bin [2 ]
Huebner, Rene [3 ]
Luo, Yunjun [1 ]
Du, Ran [1 ]
机构
[1] Beijing Inst Technol, Minist Educ, Sch Mat Sci & Engn, Key Lab High Energy Dens Mat, Beijing 100081, Peoples R China
[2] Shandong Univ, Sch Chem & Chem Engn, Jinan 250100, Peoples R China
[3] Helmholtz Zent Dresden Rossendorf, Inst Ion Beam Phys & Mat Res, Bautzner Landstr 400, D-01328 Dresden, Germany
基金
中国国家自然科学基金;
关键词
electrocatalysis; metal aerogels; sol-gel; nanostructures; porous materials; HIGH-PERFORMANCE ELECTROCATALYST; BIMETALLIC AEROGELS; OXIDATION REACTION; EVOLUTION REACTION; BUILDING-BLOCKS; CU AEROGEL; PD; AG; NANOPARTICLES; AU;
D O I
10.3390/catal13010167
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Nowadays, great efforts have been spent on addressing concerns over energy and environmental crises. Among these efforts, electrocatalysis is widely recognized and studied for its high efficiency and easy processability. As a class of emerging electrocatalysts, metal aerogels (MAs) stand out in the last decade. In virtue of their three-dimensional conductive pathways, their library of catalytically/optically active sites, and their robust network structures, MAs have unique advantages in electrocatalysis. However, due to the short history of MAs, there is insufficient research on them, leaving significant room for material design and performance optimization. This perspective will mainly focus on electrocatalysis with MAs, aiming to summarize the state-of-the-art progress and to guide the on-target design of efficient MAs-based electrocatalysts towards energy- and environment-related applications.
引用
收藏
页数:18
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[81]   Gold Aerogels: Three-Dimensional Assembly of Nanoparticles and Their Use as Electrocatalytic Interfaces [J].
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Oschatz, Martin ;
Holzschuh, Matthias ;
Wolf, Andre ;
Simon, Frank ;
Kaskel, Stefan ;
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ACS NANO, 2016, 10 (02) :2559-2567
[82]   A Membraneless Glucose/O2 Biofuel Cell Based on Pd Aerogels [J].
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[83]   Controlling the Growth of Palladium Aerogels with High-Performance toward Bioelectrocatalytic Oxidation of Glucose [J].
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[85]   Engineering Bismuth-Tin Interface in Bimetallic Aerogel with a 3D Porous Structure for Highly Selective Electrocatalytic CO2 Reduction to HCOOH [J].
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Wu, Hengbo ;
Cai, Weiquan ;
Wen, Zhenhai ;
Jia, Baohua ;
Wang, Lei ;
Jin, Wei ;
Ma, Tianyi .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2021, 60 (22) :12554-12559
[86]   Ultrasmall Gold Nanoclusters-Enabled Fabrication of Ultrafine Gold Aerogels as Novel Self-Supported Nanozymes [J].
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Wen, Dan ;
Shang, Li .
SMALL, 2022, 18 (21)
[87]   Cooperativity of Cu and Pd active sites in CuPd aerogels enhances nitrate electroreduction to ammonia [J].
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Yazdan-Abad, Mehdi Zareie ;
Noroozifar, Meissam ;
Douk, Abdollatif Shafaei ;
Modarresi-Alam, Ali Reza ;
Saravani, Hamideh .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2019, 250 :242-249