Properties-activity correlation of Nickel supported on fibrous Zeolite-Y for dry reforming of methane

被引：15

作者：

Miskan, S. N. ^{[1
]}

Setiabudi, H. D. ^{[1
,2
]}

Bahari, M. B. ^{[3
]}

Vo, Dai-Viet N. ^{[4
]}

Abdullah, B. ^{[5
]}

Jalil, A. A. ^{[6
]}

Muhammad, S. A. F. Syed ^{[7
]}

Ismail, S. B. ^{[8
]}

机构：

[1] Univ Malaysia Pahang, Fac Chem & Proc Engn Technol, Lebuhraya Tun Razak, Gambang Kuantan 26300, Pahang, Malaysia

[2] Univ Malaysia Pahang, Ctr Res Adv Fluid & Proc, Kuantan 26300, Pahang, Malaysia

[3] Univ Teknol Malaysia, Fac Sci, Skudai 81310, Johor, Malaysia

[4] Nguyen Tat Thanh Univ, Ctr Excellence Green Energy & Environm Nanomat CE@, 300 A Nguyen Tat Thanh, Ho Chi Minh City 755414, Vietnam

[5] Univ Teknol PETRONAS, Dept Chem Engn, Bandar Seri Iskanda 32610, Perak, Malaysia

[6] Univ Teknol Malaysia, Inst Future Energy, Ctr Hydrogen Energy, Skudai 81310, Johor, Malaysia

[7] Univ Teknol Malaysia, Fac Chem & Energy Engn, Bioproc & Polymer Engn Dept, Utm Skudai 81310, Johor Bahru, Malaysia

[8] Univ Malaysia Terengganu, Fac Ocean Engn Technol & Informat, Kuala Nerus 21030, Malaysia

来源：

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY | 2024年 / 52卷

关键词：

Fibrous; Zeolite-Y; Ni-based catalyst; Dry reforming of methane; Hydrogen; NI CATALYSTS; HYDROGEN; ZSM-5;

D O I：

10.1016/j.ijhydene.2022.12.201

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Nickel-supported Fibrous zeolite-Y (Ni/FHY) was successfully synthesized via the micro-emulsion method using HY as seed, followed by catalytic evaluation in dry reforming of methane (DRM) for hydrogen production. Ni/FHY possessed good NiO distribution, improved metal-support interface, and strong basicity, accredited to the fibrous structure of FHY. This unique morphology led to the enrichment in the amount of accessible Ni active sites, thus resulting in the superior activity of Ni/FHY (XCH4 = 95:1% ; XCO2 = 91.1% , H2/CO = 0.89) compared to Ni/HY (XCH4 = 92.7%, XCO2 = 89.8% ,H2/CO = 0.78). Meanwhile, the inferior performance of Ni/HY could be caused by the poor distribution of Ni with large particles, thus contributing to high carbon deposition and Ni sintering. The unique physicochemical properties and superior catalytic activity confirmed its viability in the DRM.(c) 2022 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

引用

页码：268 / 277

页数：10

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