(La0.2Dy0.2Nd0.2Sm0.2Eu0.2)2GdTaO7: a promising candidate oxides for high-temperature coating applications

被引:2
作者
Zhang, Haoming [1 ]
Zhang, Hongsong [1 ]
Liu, Shuaixia [2 ]
Zhang, Xianping [3 ]
Chen, Xiaoge [3 ]
Wang, Hong [3 ]
Wang, Yinghui [3 ]
Duan, Huanlin [3 ]
Xue, Yongfei [3 ]
机构
[1] Henan Univ Engn, Dept Mech Engn, Zhengzhou 451191, Peoples R China
[2] Henan Univ Engn, Dept Environm & Biol Engn, Zhengzhou 451191, Peoples R China
[3] Henan Univ Engn, Dept Civil Engn, Zhengzhou 451191, Peoples R China
来源
JOURNAL OF MATERIALS RESEARCH AND TECHNOLOGY-JMR&T | 2023年 / 25卷
关键词
High-temperature coatings; High-entropy oxide; Rare earth tantalum oxide; properties; Thermophysical and mechanical; THERMAL BARRIER COATINGS; MECHANICAL-PROPERTIES; CONDUCTIVITY;
D O I
10.1016/j.jmrt.2023.06.256
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
In the paper, the (La0.2Dy0.2Nd0.2Sm0.2Eu0.2)2GdTaO7 oxide was prepared employing sol-gel and solid-reaction method. Its crystal-structure, microstructure, element-distribution, mechanical and thermophysical properties are investigated. The analytical conclusions reveal that this high-entropy oxide shows single pyrochlore structure, dense microstructure, and even element distribution. Owing to the strong phonon scattering originated from high-entropy effect and numerous oxygen vacancies, it has low thermal conductivity and ranges from 1.41 to 1.27 W/m. K. Its coefficient of thermal expansion is less than those of rare-earth cerium oxides and greater than that of 7YSZ. The Young's modulus of this highentropy oxide is in the same order with 7YSZ, its Vickers hardness and fracture-toughness are lower than those of 7YSZ. This high-entropy oxide is also of excellent lattice-stability up to 1200 degrees C. (c) 2023 The Authors. Published by Elsevier B.V. This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).
引用
收藏
页码:6511 / 6523
页数:13
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