Fabrication of 3D ordered mesoporous nickel phosphide for efficient hydrogen evolution reaction

被引：6
|
作者：
Zhao, Xixi [1 ]
Wu, Wenzhe [1 ]
Gai, Hengjun [1 ]
Song, Hongbing [1 ]
Xiao, Meng [1 ]
Zhu, Quanhong [1 ]
Liang, Jilei [2 ]
Huang, Tingting [1 ]
机构：
[1] Qingdao Univ Sci & Technol, Coll Chem Engn, State Key Lab Base Ecochem Engn, Qingdao 266042, Peoples R China
[2] Taizhou Univ, Coll Pharm & Chem & Chem Engn, Taizhou 225300, Peoples R China
来源：
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY | 2023年 / 48卷 / 08期
基金：
中国国家自然科学基金;
关键词：
Ordered mesopores; Nickel phosphide; Electrocatalysis; Hydrogen production; NANOSHEET ARRAYS; OXYGEN REDUCTION; HIGH-PERFORMANCE; FACILE SYNTHESIS; ELECTROCATALYST; SURFACE; MOS2; CATALYSTS; NANOCRYSTALS; NANORODS;
D O I：
10.1016/j.ijhydene.2022.10.180
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
This article successfully fabricates ordered mesoporous nickel phosphide (OM-Ni2P) by a nanocasting method using KIT-6 as the template and nickel nitrate as the nickel precursor. The synthesized OM-Ni2P catalyst perfectly repeats the highly symmetrical mesoporous structure of KIT-6 and exhibits a large amount of the active Ni substance Ni delta+ and the active P substance P delta-. The ordered mesoporous structure not only promotes electron transfer but also facilitates the diffusion of the reaction medium. OM-Ni2P shows superior hydrogen evolution reaction (HER) electrocatalytic performance than the CA-Ni2P catalyst with a disordered mesoporous structure. The OM-Ni2P material is promising to be a sub-stitute to Pt-based electrocatalysts for hydrolysis. (c) 2022 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码：3013 / 3025
页数：13
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