Stable continuous-wave lasing from discrete cesium lead bromide quantum dots embedded in a microcavity

被引:9
作者
Zhang, Hongbo [1 ]
Wen, Wen [1 ]
Du, Bowen [1 ,4 ]
Zhou, Lei [6 ]
Chen, Yu [1 ,7 ]
Feng, Shun [1 ,8 ]
Zou, Chenji [1 ]
Wu, Lishu [1 ]
Fan, Hong Jin [1 ]
Gao, Weibo [1 ]
Sun, Handong [1 ]
Shang, Jingzhi [5 ]
Yu, Ting [2 ,3 ]
机构
[1] Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore
[2] Wuhan Univ, Sch Phys Sci & Technol, Wuhan 430072, Peoples R China
[3] Wuhan Inst Quantum Technol, Wuhan 430206, Peoples R China
[4] Shenzhen Univ, Coll Phys & Optoelect Engn, Shenzhen 518060, Peoples R China
[5] Northwestern Polytech Univ, Shaanxi Inst Flexible Elect SIFE, Xian 710129, Peoples R China
[6] Sun Yat Sen Univ, Sch Chem Engn & Technol, Zhuhai 519082, Peoples R China
[7] Commonwealth Sci & Ind Res Org CSIRO Mfg, Clayton, Vic 3168, Australia
[8] Heriot Watt Univ, Inst Photon & Quantum Sci, SUPA, Edinburgh EH14 4AS, Scotland
基金
欧盟地平线“2020”; 新加坡国家研究基金会;
关键词
SINGLE-PHOTON EMISSION; PEROVSKITE; CSPBBR3; LASERS;
D O I
10.1039/d3nh00139c
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
All-inorganic cesium lead bromide (CsPbBr3) quantum dots (QDs) with high photoluminescence (PL) quantum efficiency have been reported as ideal gain materials for high-performance lasers. Nevertheless, isolated CsPbBr3 QDs have not achieved lasing emission (LE) due to finite absorption cross-section. Here, we demonstrate continuous-wave lasing of isolated CsPbBr3 QDs embedded in a microcavity. Distributed Bragg reflectors (DBRs), together with isolated CsPbBr3 QDs in a polymer matrix, are introduced to construct a vertical-cavity surface-emitting laser (VCSEL), which exhibits stable single-mode lasing emissions with an ultra-low threshold of 8.8 W cm(-2) and a high Q factor of 1787. Such perovskite-based microcavity structures sustain highly stable excitons at room temperature and can provide an excellent experimental platform to further study the single-particle nano-lasers and quantum physics frontiers such as exciton-polariton condensation, single-photon emission, and optical quantum communication.
引用
收藏
页码:1403 / 1410
页数:8
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