High-performance aqueous zinc-ion hybrid capacitors based on 3D printed metal-organic framework cathodes

被引：34

作者：

Catarineu, Noelle R. ^{[1
]}

Lin, Dun ^{[2
]}

Zhu, Cheng ^{[1
]}

Oyarzun, Diego I. ^{[1
]}

Li, Yat ^{[2
]}

机构：

[1] Lawrence Livermore Natl Lab, Lab Energy Applicat Future LEAF, Livermore, CA 94550 USA

[2] Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA

来源：

CHEMICAL ENGINEERING JOURNAL | 2023年 / 465卷

关键词：

CARBON AEROGELS; POROUS CARBON; STORAGE; STABILITY; SUPERCAPACITOR; REINFORCEMENT; ADSORPTION; ELECTRODES; INNER;

D O I：

10.1016/j.cej.2023.142544

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

The zinc-ion hybrid capacitor is a promising energy storage device, but current overall capacity is limited by the capacitance of the carbon cathode. We produced a hierarchically porous, nitrogen-doped carbon cathode with good cycling and mechanical stability by 3D printing and pyrolysis of the zinc-based metal-organic framework ZIF-8. When incorporated into a zinc-ion hybrid capacitor, we achieved an areal capacitance of 16.9 F cm-2 and energy density of 7.23 mW h cm-2, outperforming zinc-ion hybrid capacitors based on conventional cathodes.

引用

页数：10

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