Aircraft emissions;
Pollutants;
Ultrafine particles;
Public health;
Turbulent mixing;
ULTRAFINE PARTICLE CONCENTRATIONS;
ANGELES-INTERNATIONAL-AIRPORT;
NUMBER CONCENTRATIONS;
AIRCRAFT;
EMISSIONS;
URBAN;
D O I:
10.1016/j.apr.2023.101696
中图分类号:
X [环境科学、安全科学];
学科分类号:
08 ;
0830 ;
摘要:
Despite ample evidence that pollutant emissions from aircraft may cause or exacerbate human health problems and have considerable environmental impacts, ambient air quality measurements including particle number size distributions (PNSD) near airports are scarce. We performed two measurement campaigns of particulate (ultrafine particles (UFP) and PM1.0, PM2.5, PM10) and gaseous (NO, NO2, O3) pollutants near a mid-sized airport in Central Europe (Findel, Luxembourg) during summer 2018 and winter/spring 2019. Mean UFP number concentrations (5-350 nm) were dominated by nucleation mode particles that are one of the major environmental health risks in Europe. Mean values during summer (-9200 # cm-3) exceeded those measured during winter (-7800 # cm-3). PNSD maxima of UFP occurred at sizes of 12.6 nm in the summer and 14.6 nm in the winter when air masses arrived from the airport sector to the measurement site. K-means cluster analysis revealed that air masses arriving from forest or urban background sectors are characterized by an UFP signal that is a factor of five to 10 lower than of the airport sector. During the winter/spring season the main airport NO2 (and PM2.5) emissions are attributed to exhaust gases from heating systems of airport buildings. Pollutant concentrations (except O3), including UFP were diminished during daytime due to turbulent mixing, although flight movements were highest during that time. This study presents a new perspective on the critical role of mixed layer temporal dynamics on the dilution of pollutant and UFP concentrations that is influenced by airport siting and terrain.
机构:
Harvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USAHarvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USA
Hsu, Hsiao-Hsien
Adamkiewicz, Gary
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Harvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USAHarvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USA
Adamkiewicz, Gary
Houseman, E. Andres
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Harvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USA
Brown Univ, Warren Alpert Med Sch, Providence, RI 02912 USAHarvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USA
Houseman, E. Andres
Vallarino, Jose
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Harvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USAHarvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USA
Vallarino, Jose
Melly, Steven J.
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Harvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USAHarvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USA
Melly, Steven J.
Wayson, Roger L.
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Volpe Natl Transportat Syst Ctr, Cambridge, MA 02142 USAHarvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USA
Wayson, Roger L.
Spengler, John D.
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Harvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USAHarvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USA
Spengler, John D.
Levy, Jonathan I.
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Harvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USA
Boston Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02118 USAHarvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USA
机构:
Icahn Sch Med Mt Sinai, Dept Prevent Med, Ctr Adv Med, New York, NY 10029 USAIcahn Sch Med Mt Sinai, Dept Prevent Med, Ctr Adv Med, New York, NY 10029 USA
Hsu, Hsiao-Hsien
Adamkiewicz, Gary
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Harvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USAIcahn Sch Med Mt Sinai, Dept Prevent Med, Ctr Adv Med, New York, NY 10029 USA
Adamkiewicz, Gary
Houseman, E. Andres
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h-index: 0
机构:
Harvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USA
Oregon State Univ, Coll Publ Hlth & Human Sci, Corvallis, OR 97331 USAIcahn Sch Med Mt Sinai, Dept Prevent Med, Ctr Adv Med, New York, NY 10029 USA
Houseman, E. Andres
Spengler, John D.
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h-index: 0
机构:
Harvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USAIcahn Sch Med Mt Sinai, Dept Prevent Med, Ctr Adv Med, New York, NY 10029 USA
Spengler, John D.
Levy, Jonathan I.
论文数: 0引用数: 0
h-index: 0
机构:
Harvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02215 USA
Boston Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02118 USAIcahn Sch Med Mt Sinai, Dept Prevent Med, Ctr Adv Med, New York, NY 10029 USA
机构:
Italian Natl Res Council CNR, Inst Atmospher Pollut Res, I-00016 Rome, ItalyItalian Natl Res Council CNR, Inst Atmospher Pollut Res, I-00016 Rome, Italy
Vichi, Francesca
Frattoni, Massimiliano
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Italian Natl Res Council CNR, Inst Atmospher Pollut Res, I-00016 Rome, ItalyItalian Natl Res Council CNR, Inst Atmospher Pollut Res, I-00016 Rome, Italy
Frattoni, Massimiliano
Imperiali, Andrea
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Italian Natl Res Council CNR, Inst Atmospher Pollut Res, I-00016 Rome, ItalyItalian Natl Res Council CNR, Inst Atmospher Pollut Res, I-00016 Rome, Italy
Imperiali, Andrea
Balducci, Catia
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Italian Natl Res Council CNR, Inst Atmospher Pollut Res, I-00016 Rome, ItalyItalian Natl Res Council CNR, Inst Atmospher Pollut Res, I-00016 Rome, Italy
Balducci, Catia
Cecinato, Angelo
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Italian Natl Res Council CNR, Inst Atmospher Pollut Res, I-00016 Rome, ItalyItalian Natl Res Council CNR, Inst Atmospher Pollut Res, I-00016 Rome, Italy
Cecinato, Angelo
Perilli, Mattia
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Italian Natl Res Council CNR, Inst Atmospher Pollut Res, I-00016 Rome, ItalyItalian Natl Res Council CNR, Inst Atmospher Pollut Res, I-00016 Rome, Italy
Perilli, Mattia
Romagnoli, Paola
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Italian Natl Res Council CNR, Inst Atmospher Pollut Res, I-00016 Rome, ItalyItalian Natl Res Council CNR, Inst Atmospher Pollut Res, I-00016 Rome, Italy