Static and dynamical properties of the spin-52 nearly ideal triangular lattice antiferromagnet Ba3MnSb2O9

被引:5
作者
Shu, Mingfang [1 ,2 ]
Dong, Weicen [1 ,2 ]
Jiao, Jinlong [1 ,2 ]
Wu, Jiangtao [1 ,2 ]
Lin, Gaoting [1 ,2 ]
Kamiya, Yoshitomo [1 ,2 ]
Hong, Tao [3 ]
Cao, Huibo [3 ]
Matsuda, Masaaki [3 ]
Tian, Wei [3 ]
Chi, Songxue [3 ]
Ehlers, G. [3 ]
Ouyang, Zhongwen [4 ]
Chen, Hongwei [5 ,7 ]
Zou, Youming [5 ]
Qu, Zhe [5 ]
Huang, Qing [6 ,8 ]
Zhou, Haidong [6 ]
Ma, Jie [1 ,2 ,4 ]
机构
[1] Shanghai Jiao Tong Univ, Sch Phys & Astron, Key Lab Artificial Struct & Quantum Control, Shanghai 200240, Peoples R China
[2] Nanjing Univ, Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Jiangsu, Peoples R China
[3] Oak Ridge Natl Lab, Neutron Scattering Div, Oak Ridge, TN 37831 USA
[4] Huazhong Univ Sci & Technol, Wuhan Natl High Magnet Field Ctr, Wuhan 430074, Peoples R China
[5] Chinese Acad Sci, Hefei Inst Phys Sci, Anhui Key Lab Condensed Matter Phys Extreme Condit, High Magnet Field Lab, Hefei 230031, Anhui, Peoples R China
[6] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA
[7] China Jiliang Univ, Coll Mat Sci & Chem, Hangzhou 310018, Peoples R China
[8] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA
基金
美国国家科学基金会;
关键词
HIGH-FIELD MAGNETIZATION; HEISENBERG-ANTIFERROMAGNET; EXCITATIONS; DIAGONALIZATION; RESONANCE; PHASE; ESR;
D O I
10.1103/PhysRevB.108.174424
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We study the ground state and spin excitations in Ba3MnSb2O9, an easy-plane S = 5/2 triangular lattice antiferromagnet. By combining single-crystal neutron scattering, electric spin resonance (ESR), and spin wave calculations, we determine the frustrated quasi-two-dimensional spin Hamiltonian parameters describing the material. While the material has a slight monoclinic structural distortion, which could allow for isoscelestriangular exchanges and biaxial anisotropy by symmetry, we observe no deviation from the behavior expected for spin waves in the in-plane 120 degrees state. Even the easy-plane anisotropy is so small that it can only be detected by ESR in our study. In conjunction with the quasitwo dimensionality, our study establishes that Ba3MnSb2O9 is a nearly ideal triangular lattice antiferromagnet with the quasiclassical spin S = 5/2, which suggests that it has the potential for an experimental study of Z- or Z2-vortex excitations.
引用
收藏
页数:12
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共 63 条
  • [1] RESONATING VALENCE BONDS - NEW KIND OF INSULATOR
    ANDERSON, PW
    [J]. MATERIALS RESEARCH BULLETIN, 1973, 8 (02) : 153 - 160
  • [2] Spin Current as a Probe of the Z2-Vortex Topological Transition in the Classical Heisenberg Antiferromagnet on the Triangular Lattice
    Aoyama, K.
    Kawamura, H.
    [J]. PHYSICAL REVIEW LETTERS, 2020, 124 (04)
  • [3] Spin liquids in frustrated magnets
    Balents, Leon
    [J]. NATURE, 2010, 464 (7286) : 199 - 208
  • [4] Chakoumakos BC, 2011, J APPL CRYSTALLOGR, V44, P655, DOI [10.1107/S0021889811012301, 10.1107/S0021889811012301655]
  • [5] Spin waves in a triangular lattice antiferromagnet: Decays, spectrum renormalization, and singularities
    Chernyshev, A. L.
    Zhitomirsky, M. E.
    [J]. PHYSICAL REVIEW B, 2009, 79 (14):
  • [6] Magnon decay in noncollinear quantum antiferromagnets
    Chernyshev, A. L.
    Zhitomirsky, M. E.
    [J]. PHYSICAL REVIEW LETTERS, 2006, 97 (20)
  • [7] Spin Excitation Spectra of Anisotropic Spin-1/2 Triangular Lattice Heisenberg Antiferromagnets
    Chi, Runze
    Liu, Yang
    Wan, Yuan
    Liao, Hai-Jun
    Xiang, T.
    [J]. PHYSICAL REVIEW LETTERS, 2022, 129 (22)
  • [8] UNIVERSAL MAGNETIC-PROPERTIES OF FRUSTRATED QUANTUM ANTIFERROMAGNETS IN 2 DIMENSIONS
    CHUBUKOV, AV
    SENTHIL, T
    SACHDEV, S
    [J]. PHYSICAL REVIEW LETTERS, 1994, 72 (13) : 2089 - 2092
  • [9] QUANTUM-THEORY OF AN ANTIFERROMAGNET ON A TRIANGULAR LATTICE IN A MAGNETIC-FIELD
    CHUBUKOV, AV
    GOLOSOV, DI
    [J]. JOURNAL OF PHYSICS-CONDENSED MATTER, 1991, 3 (01) : 69 - 82
  • [10] Extended scattering continua characteristic of spin fractionalization in the two-dimensional frustrated quantum magnet Cs2CuCl4 observed by neutron scattering -: art. no. 134424
    Coldea, R
    Tennant, DA
    Tylczynski, Z
    [J]. PHYSICAL REVIEW B, 2003, 68 (13)