PVDF membrane with tea powder adhered for efficient separation of emulsified oil

被引:6
作者
Zhang, Junshuang [1 ]
Wu, Yue [1 ]
Xia, Mengsheng [2 ]
Yang, Qijiang [1 ]
Xu, Qinyao [2 ]
Feng, Wenwen [3 ]
机构
[1] Guangzhou Maritime Univ, Sch Marine Engn, 101 Hongshan Third Rd, Guangzhou 510725, Peoples R China
[2] Zhejiang Ocean Univ, Sch Ships & Maritime Transport, 1 Haida South Rd, Zhoushan City 316022, Peoples R China
[3] Guangdong Ind Polytech, Sch Light Chem Technol, 152 Xingang West Rd, Guangzhou City 510300, Peoples R China
关键词
Super Wetting Materials; Tea Powder; PVDF Membrane; Oil-in-water Emulsions; Separation; IN-WATER EMULSIONS; COATED MEMBRANES; PERFORMANCE; POLLUTION;
D O I
10.1007/s11814-023-1541-9
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Conventional oily wastewater treatment can remove slick oil and dispersed oil well, but it is difficult for it to remove emulsified oil. Nonetheless, the development of super wetting materials provides a key role in treating the emulsified oil, but there are some problems, such as expensive raw materials, complicated processes, as well as secondary pollution. In order to treat these problems, a brand-new oil/water separation membrane (TEA/PVDF membrane) was developed by combining the viscosity of sodium alginate (SA) and the filter tea powder (TEA) onto the surface of the polyvinylidene fluoride (PVDF) membrane by a vacuum pump. Furthermore, the underwater oleophobic angle reached 135o. Moreover, the oil-water separation experiments of oil-in-water emulsion utilizing TEA/PVDF membrane demonstrated excellent separation efficiency (99.6%) and good flux (254 L m-2 h-1 bar-1). Notably, upon ten cycles, the oil removal rate was still as high as 99.2%. Moreover, the TEA/PVDF membrane was able to separate oil-in-water emulsions in environments with strong acids, strong bases, and high salt concentrations, with a separation efficiency of over 95.9%. Such a novel oil/water separation membrane is economic, environmentally protective, and simple production process, which exhibits overwhelming potential in practical life for treating oily wastewater.
引用
收藏
页码:2376 / 2383
页数:8
相关论文
共 50 条
[21]   Fabrication of modified PVDF membranes with PAA network polymer for highly efficient oil/water emulsion separation [J].
Zhao, Chen ;
Wang, ShanShan ;
Wang, Nianping .
SEPARATION AND PURIFICATION TECHNOLOGY, 2025, 357
[22]   A mussel inspired highly stable graphene oxide membrane for efficient oil-in-water emulsions separation [J].
Liu, Zhanchao ;
Wu, Weifu ;
Liu, Yan ;
Qin, Changchun ;
Meng, Minjia ;
Jiang, Yinhua ;
Qiu, Jian ;
Peng, Jianbo .
SEPARATION AND PURIFICATION TECHNOLOGY, 2018, 199 :37-46
[23]   Fabrication of crosslinking modified PVDF/GO membrane with acid, alkali and salt resistance for efficient oil-water emulsion separation [J].
Cui, Jiuyun ;
Xie, Atian ;
Yan, Zhuo ;
Yan, Yongsheng .
SEPARATION AND PURIFICATION TECHNOLOGY, 2021, 265
[24]   Pine powders-coated PVDF multifunctional membrane for highly efficient switchable oil/water emulsions separation and dyes adsorption [J].
Wu, Mingming ;
Mu, Peng ;
Li, Bingfeng ;
Wang, Qingtao ;
Yang, Yaoxia ;
Li, Jian .
SEPARATION AND PURIFICATION TECHNOLOGY, 2020, 248
[25]   Surface morphology of pvdf membrane and its fouling phenomenon by crude oil emulsion [J].
Susan, L. Y. ;
Ismail, S. ;
Ooi, B. S. ;
Mustapa, H. .
JOURNAL OF WATER PROCESS ENGINEERING, 2017, 15 :55-61
[26]   One-pot Synthesis of Multifunctional KGM/PDA/PVDF Composite Membrane for Efficient Treatment of Oil-water Emulsion and Dye [J].
Wu, Yilin ;
Yan, Yan ;
Lu, Jian ;
Yu, Zhixin ;
Wu, Junda ;
Wang, Qianqian ;
Jiang, Zhongyi .
NANO, 2021, 16 (03)
[27]   An Intelligent Superwetting PVDF Membrane Showing Switchable Transport Performance for Oil/Water Separation [J].
Tao, Mimi ;
Xue, Lixin ;
Liu, Fu ;
Jiang, Lei .
ADVANCED MATERIALS, 2014, 26 (18) :2943-2948
[28]   Dialdehyde cellulose (DAC) and polyethyleneimine (PEI) coated polyvinylidene fluoride (PVDF) membrane for simultaneously removing emulsified oils and anionic dyes [J].
Liu, Junliang ;
Huang, Yixuan ;
Zhang, Ganwei ;
Wang, Qianhui ;
Shen, Shusu ;
Liu, Dapeng ;
Hong, Yaoliang ;
Wyman, Ian .
JOURNAL OF HAZARDOUS MATERIALS, 2024, 471
[29]   Purification of emulsified oil by Bentonite loaded polyvinylidene fluoride/polyvinylpyrrolidone membrane [J].
Nigiz, F. U. ;
Yucak, A. I. ;
Hilmioglu, N. D. .
WATER PRACTICE AND TECHNOLOGY, 2020, 15 (02) :394-403
[30]   Tailoring Morphology of PVDF-HFP Membrane via One-step Reactive Vapor Induced Phase Separation for Efficient Oil-Water Separation [J].
Huo, Peng ;
Zhong, Cheng-Tang ;
Xiong, Xiao-Peng .
CHINESE JOURNAL OF POLYMER SCIENCE, 2021, 39 (05) :610-619