In-situ visualization of cathode flow channel in polymer electrolyte membrane fuel cell: Effect of GDL degradation

被引:5
|
作者
Moon, Jong Woon [1 ]
Kim, Seong Keun [1 ]
Jung, Sung Yong [1 ]
机构
[1] Chosun Univ, Dept Mech Engn, 10 Chosundae 1-Gil, Gwangju 61452, South Korea
关键词
PEMFC; GDL; In-situ flow visualization; Two-phase flow; WATER MANAGEMENT;
D O I
10.1016/j.ijhydene.2023.03.342
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Polymer electrolyte membrane fuel cells (PEMFCs) are used in various fields, but their lifetime should be considered for commercial applications. The degradation of their gas diffusion layer (GDL), which enables fuel diffusion and water management, can reduce the performance and accelerate the degradation of other components. This study investigates the effect of GDL degradation on in-situ flow characteristics in cathode flow channels. A special cell is designed to visualize in-situ two-phase flows in the cathode flow channel with a high-speed camera. As the GDL degrades, the flow pattern changes from dropwise to slug and annular flows. Moreover, the amount of residual liquid after one water discharge cycle increases as the GDL deteriorates. These changes in the flow patterns and remaining liquid can disrupt the fuel supply to chemical reaction sites and degrade PEMFC performance.(c) 2023 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:1255 / 1263
页数:9
相关论文
共 50 条
  • [21] Effect of convective channel-to-channel mass flow in a polymer electrolyte fuel cell
    von Dahlen, S.
    Bayer, M. H.
    Schneider, I. A.
    ELECTROCHEMISTRY COMMUNICATIONS, 2012, 14 (01) : 55 - 58
  • [22] EFFECTS OF WETTABILITY AND FLOW DIRECTION OF CATHODE CHANNEL ON PLUGGING PHENOMENON IN POLYMER ELECTROLYTE FUEL CELL
    Taniguchi, Ryo
    Nishida, Kosuke
    Kamada, Hisashi
    Tsushima, Shohji
    Hirai, Shuichiro
    PROCEEDINGS OF THE ASME 9TH INTERNATIONAL CONFERENCE ON FUEL CELL SCIENCE, ENGINEERING, AND TECHNOLOGY 2011, 2012, : 181 - 186
  • [23] Numerical analysis on performances of polymer electrolyte membrane fuel cells with various cathode flow channel geometries
    Wang, Xiao-Dong
    Lu, Gui
    Duan, Yuan-Yuan
    Lee, Duu-Jong
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2012, 37 (20) : 15778 - 15786
  • [24] Advantages and disadvantages of various cathode flow field designs for a polymer electrolyte membrane fuel cell
    Lim, Kisung
    Vaz, Neil
    Lee, Jaeseung
    Ju, Hyunchul
    INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER, 2020, 163
  • [25] New design of a cathode flow-field with a sub-channel to improve the polymer electrolyte membrane fuel cell performance
    Wang, Yulin
    Yue, Like
    Wang, Shixue
    JOURNAL OF POWER SOURCES, 2017, 344 : 32 - 38
  • [26] The influence of polymer electrolyte fuel cell cathode degradation on the electrode polarization
    Aoki, Tsutomu
    Matsunaga, Atsushi
    Ogami, Yasuji
    Maekawa, Akira
    Mitsushima, Shigenori
    Ota, Ken-ichiro
    Nishikawa, Hisao
    JOURNAL OF POWER SOURCES, 2010, 195 (08) : 2182 - 2188
  • [27] Operando 3D Visualization of Migration and Degradation of a Platinum Cathode Catalyst in a Polymer Electrolyte Fuel Cell
    Matsui, Hirosuke
    Ishiguro, Nozomu
    Uruga, Tomoya
    Sekizawa, Oki
    Higashi, Kotaro
    Maejima, Naoyuki
    Tada, Mizuki
    ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2017, 56 (32) : 9371 - 9375
  • [28] Degradation of polymer electrolyte membrane fuel cell by siloxane in biogas
    Seo, Ji-Sung
    Kim, Da-Yeong
    Hwang, Sun-Mi
    Seo, Min Ho
    Seo, Dong-Jun
    Yang, Seung Yong
    Han, Chan Hui
    Jung, Yong-Min
    Guim, Hwanuk
    Nahm, Kee Suk
    Yoon, Young-Gi
    Kim, Tae Young
    JOURNAL OF POWER SOURCES, 2016, 316 : 44 - 52
  • [29] Polymer electrolyte membrane fuel cell contamination: Testing and diagnosis of toluene-induced cathode degradation
    Li, Hui
    Zhang, Jianlu
    Fatih, Khalid
    Wang, Zhenwei
    Tang, Yanghua
    Shi, Zheng
    Wu, Shaohong
    Song, Datong
    Zhang, Jiujun
    Jia, Nengyou
    Wessel, Silvia
    Abouatallah, Rami
    Joos, Nathan
    JOURNAL OF POWER SOURCES, 2008, 185 (01) : 272 - 279
  • [30] Study on accelerated stress test and degradation for open cathode stack in polymer electrolyte membrane fuel cell
    Yoo, Donggeun
    Park, Kwonpil
    JOURNAL OF POWER SOURCES, 2024, 624