Zeolite supported CdS/TiO2/CeO2 composite: Synthesis, characterization and photocatalytic activity for methylene blue dye degradation

被引:41
|
作者
Mahamud, Mohammedsani [1 ]
Taddesse, Abi M. [1 ]
Bogale, Yiheyis [1 ]
Bezu, Zewdu [1 ]
机构
[1] Haramaya Univ, Coll Nat & Computat Sci, Dept Chem, Dire Dawa, Ethiopia
关键词
Degradation; Zeolite; Composite; Photocatalysis; Wastewater; Visible light; TIO2; REMOVAL;
D O I
10.1016/j.materresbull.2023.112176
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
A novel ternary composite CdS/TiO2/CeO2 and its zeolite-support were synthesized and characterized using XRD, SEM, UV-Vis DRS and PL spectroscopy. The photocatalytic performance of the synthesized nanocomposites was investigated using an aqueous solution of Methylene Blue (MB) dye and a real sewage sample solution.The photocatalytic activity of the zeolite-supported composite was superior to the naked CdS/TiO2/CeO2, binary, and single counter constituents. The effect of operational parameters on MB dye degradation was evaluated, and a significant photodegradation was recorded by a zeolite-supported CdS/TiO2/CeO2 composite. The supported composite showed significantly higher performance on the discoloration of MB (99.9%) than the real sewage sample solution (78.7%) based on the optimized parameters. The recyclability study of the spent photocatalyst exhibited 86.0% degradation of MB after four consecutive cycles, indicating the stability of the composite. Based on the findings, this research offers insight into a new and efficient visible-light-driven photocatalyst for the degradation of organic dyes in wastewater.
引用
收藏
页数:11
相关论文
共 50 条
  • [11] Electrospun TiO2 Microspheres with Enhanced Activity for Photocatalytic Degradation of Methylene Blue
    Zhang, Hong
    Liu, Xinjuan
    Sun, Zhuo
    ASIAN JOURNAL OF CHEMISTRY, 2013, 25 (12) : 6963 - 6967
  • [12] Integration of Adsorption and Photocatalytic Degradation of Methylene Blue Using TiO2 Supported on Granular Activated Carbon
    Atout, H.
    Bouguettoucha, A.
    Chebli, D.
    Gatica, J. M.
    Vidal, H.
    Yeste, M. Pilar
    Amrane, A.
    ARABIAN JOURNAL FOR SCIENCE AND ENGINEERING, 2017, 42 (04) : 1475 - 1486
  • [13] Photocatalytic Degradation of Methylene Blue from Aqueous Solutions by rGO/TiO2 Nanocomposites
    Gao, Wei
    Li, Yufeng
    Zhao, Jitao
    Zhang, Zhe
    Tang, Weiwei
    Wang, Jun
    Wu, Zhenyu
    WATER AIR AND SOIL POLLUTION, 2023, 234 (07)
  • [14] Synthesis of Ag decorated TiO2 nanoneedles for photocatalytic degradation of methylene blue dye
    Ridha, Noor J.
    Alosfur, Firas K. Mohamad
    Kadhim, Hiba Basim Abbas
    Ahmed, Luma M.
    MATERIALS RESEARCH EXPRESS, 2021, 8 (12)
  • [15] Effect of TiO2 phase on the photocatalytic degradation of methylene blue dye
    Tichapondwa, S. M.
    Newman, J. P.
    Kubheka, O.
    PHYSICS AND CHEMISTRY OF THE EARTH, 2020, 118 (118-119)
  • [16] Preparation and Characterization of Sulfated TiO2/Zeolite Composite Catalysts with Enhanced Photocatalytic Activity
    Zhao, Yuan
    Li, JingXiu
    Wang, Ling
    Hao, Yanan
    Yang, Lin
    He, Pingting
    Xue, JianJun
    NANO, 2018, 13 (10)
  • [17] Synthesis and Photocatlytic Application of Drinking Water Treatment Sludge @ TiO2 Composite for Degradation of Methylene Blue Dye
    Rashed, M. N.
    El Taher, M. A.
    Fadlalla, S. M. M.
    POLLUTION, 2020, 6 (04): : 785 - 799
  • [18] Photocatalytic Degradation Performance of TiO2/PTFE Membrane Catalyst to Methylene Blue
    Kang, Weimin
    Ju, Jingge
    He, Hongsheng
    Li, Fu
    Tao, Liqin
    Dong, Yongchun
    Cheng, Bowen
    CHEMISTRY LETTERS, 2016, 45 (12) : 1440 - 1443
  • [19] Synthesis of TiO2/Graphene oxide nanocomposites for their enhanced photocatalytic activity against methylene blue dye and ciprofloxacin
    Khan, Shakeel Ahmad
    Arshad, Zunaira
    Shahid, Sammia
    Arshad, Ishwa
    Rizwan, Komal
    Sher, Mudassir
    Fatima, Urooj
    COMPOSITES PART B-ENGINEERING, 2019, 175
  • [20] Synthesis and characterization of CeO2 supported ZSM-5 zeolite for organic dye degradation
    Prabhu, S.
    Elumalai, N.
    Selvaraj, M.
    Harish, S.
    Ramesh, R.
    Silambarasan, A.
    Navaneethan, M.
    Ramu, P.
    JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2022, 33 (12) : 9211 - 9223