Systematically designed g-C3N4/rGO/MoS2 nanocomposite for enhanced photocatalytic performance

被引:5
作者
Sardar, Waseem [1 ]
Ali, Gohar [2 ]
Jiang, Fengchun [1 ]
Nawaz, Ahmad [3 ]
Khan, Salman [1 ]
Zubair, Muhammad [1 ]
Awan, Dawar [4 ]
Iqbal, Mahmood [5 ]
Park, Tae Joo [2 ]
机构
[1] Harbin Engn Univ, Coll Mat Sci & Chem Engn, Harbin 150001, Peoples R China
[2] Hanyang Univ ERICA, Dept Mat Sci & Chem Engn, Ansan 15588, South Korea
[3] Univ Technol, Dept Mech Engn Technol, Nowshera Kpk, Pakistan
[4] Univ Technol, Dept Energy Engn Technol, Nowshera Kpk, Pakistan
[5] Pakistan Council Sci & Ind Res Complex, Peshawar, Pakistan
关键词
rGO; MoS2; Nanocomposite; RhB degradation; ATOMIC LAYER DEPOSITION; HYDROGEN EVOLUTION; GRAPHENE OXIDE; G-C3N4; PHOTODEGRADATION; HETEROJUNCTION; NANOJUNCTION; INTERFACE; REMOVAL;
D O I
10.1016/j.cap.2023.10.015
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Two-dimensional materials like graphitic carbon nitride are gaining more interest because of their desirable features such as high thermal stability, high chemical resistance, affordability, non-toxic and non-corrosive properties. However, the recombination of photogenerated charges limits the photocatalytic efficacy g-C3N4. To address this issue, a quick and affordable hydrothermal technique was employed to create a ternary nanocomposite of molybdenum disulfide (MoS2), reduced graphene oxide (rGO), and g-C3N4 that efficiently limited charge recombination and increased photocatalytic efficiency. The synthesized g-C3N4/rGO/MoS2 nanocomposite showed enhanced photocatalytic activity due to the multi-step charge transfer mechanism and greater utilization of visible light. When compared with both pure g-C3N4 and g-C3N4/MoS2 nanocomposites, the ternary nanocomposite significantly degrades 94.1 % Rhodamine-B dye. In order to assess the properties of the nanocomposite, SEM, XPS, X-ray diffractometer, photoluminescence, and electrochemical impedance spectra were all used. This work illustrates the capability to improve dye degradation performance utilizing a simple and costeffective method.
引用
收藏
页码:42 / 48
页数:7
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