Construction of Ag/Bi2WO6/BiOCl with enhanced photocatalytic performance for efficient degradation of organic pollutant

被引：13

作者：

Wang, Haitao ^{[1
,3
]}

Shi, Baoxu ^{[1
]}

Liu, Yueqin ^{[1
]}

Guo, Jianfeng ^{[2
]}

Chang, Na ^{[2
,3
]}

Zhao, Xiaoxu ^{[1
,2
]}

机构：

[1] Tiangong Univ, Sch Environm Sci & Engn, Tianjin 300387, Peoples R China

[2] Tiangong Univ, Sch Chem Engn & Technol, Tianjin 300387, Peoples R China

[3] Tiangong Univ, State Key Lab Separat Membranes & Membrane Proc, Tianjin 300387, Peoples R China

来源：

INORGANIC CHEMISTRY COMMUNICATIONS | 2023年 / 153卷

关键词：

Bi2WO6; BiOCl; MBT; Ag NPs; Photocatalytic mechanism; BIOCL NANOSHEETS; 2-MERCAPTOBENZOTHIAZOLE; NANOPARTICLES; REDUCTION; INSIGHTS; CO2;

D O I：

10.1016/j.inoche.2023.110816

中图分类号：

O61 [无机化学];

学科分类号：

070301 ; 081704 ;

摘要：

In this study, a ternary composite photocatalyst (Ag/Bi2WO6/BiOCl) is synthesized via using hydrothermal and photo-reduction methods. The results of SEM and TEM showed that Ag/Bi2WO6/BiOCl exhibited a stacked layered structure. The Ag/Bi2WO6/BiOCl composite photocatalyst showed outstanding degradation activity of 2-mercaptobenzothiazole (MBT) under visible light, and the degradation rate reached 93.1% within 25 min, which is 3.3 and 3.9 times higher than pure Bi2WO6 and BiOCl. The synergy between Bi2WO6/BiOCl and the Ag nanoparticles (Ag NPs) effectively promoted visible light absorption and reduced the recombination efficiency of photogenerated electron-holes, indicating the enhanced photocatalytic activity of Ag/Bi2WO6/BiOCl composite photocatalyst. The possible charge transfer mechanism of Ag/Bi2WO6/BiOCl is proposed.

引用

页数：9

共 45 条

[1] Investigation of nano Ag-decorated SiC particles for photoelectrocatalytic dye degradation and bacterial inactivation [J].

Adhikari, Sangeeta ;

Eswar, Neerugatti KrishnaRao ;

Sangita, Sushree ;

Sarkar, Debasish ;

Madras, Giridhar .

JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY, 2018, 357 :118-131

[2] Facile synthesis of Co(II)-BiOCl@biochar nanosheets for photocatalytic degradation of p-nitrophenol under vacuum ultraviolet (VUV) irradiation [J].

Cao, Ting-ting ;

Cui, Han ;

Zhang, Qi-wei ;

Cui, Chong-wei .

APPLIED SURFACE SCIENCE, 2021, 559

[3] Boosted photocatalytic NO removal performance by S-scheme hierarchical composites WO3/Bi4O5Br2 prepared through a facile ball-milling protocol [J].

Chang, Fei ;

Li, Sushi ;

Shi, Zhuoli ;

Qi, Yingfei ;

Liu, Deng-guo ;

Liu, Xiaoqi ;

Chen, Shengwen .

SEPARATION AND PURIFICATION TECHNOLOGY, 2022, 278

[4] Nanostructured LaFeO3-MoS2 for efficient photodegradation and photocatalytic hydrogen evolution [J].

Das, Subrata ;

Dutta, Sagar ;

Tama, Angkita Mistry ;

Basith, M. A. .

MATERIALS SCIENCE AND ENGINEERING B-ADVANCED FUNCTIONAL SOLID-STATE MATERIALS, 2021, 271

[5] Enhanced visible-light photocatalytic degradation activity of Ti3C2/PDIsm via π-π interaction and interfacial charge separation: Experimental and theoretical investigations [J].

Duan, Mengbiao ;

Jiang, Longbo ;

Shao, Binbin ;

Feng, Chengyang ;

Yu, Hanbo ;

Guo, Hai ;

Chen, Haoyun ;

Tang, Wangwang .

APPLIED CATALYSIS B-ENVIRONMENTAL, 2021, 297

[6]

Fei Chang, 2021, Environmental Nanotechnology, Monitoring and Management, V15, P461, DOI 10.1016/j.enmm.2021.100436

[7] Bi2WO6-BiOCl heterostructure with enhanced photocatalytic activity for efficient degradation of oxytetracycline [J].

Guo, Mengfan ;

Zhou, Zhaobo ;

Yan, Shengnan ;

Zhou, Pengfei ;

Miao, Feng ;

Liang, Shijun ;

Wang, Jinlan ;

Cui, Xinyi .

SCIENTIFIC REPORTS, 2020, 10 (01)

[8] A novel Z-scheme Bi2MoO6/BiOBr photocatalyst for enhanced photocatalytic activity under visible light irradiation [J].

Hu, Taiping ;

Yang, Yang ;

Dai, Kai ;

Zhang, Jinfeng ;

Liang, Changhao .

APPLIED SURFACE SCIENCE, 2018, 456 :473-481

[9] Insights into enhanced visible light photocatalytic activity of t-Se nanorods/BiOCl ultrathin nanosheets 1D/2D heterojunctions [J].

Huang, Hai ;

Ma, Changchang ;

Zhu, Zhi ;

Yao, Xin ;

Liu, Yang ;

Liu, Zhi ;

Li, Chunxiang ;

Yan, Yongsheng .

CHEMICAL ENGINEERING JOURNAL, 2018, 338 :218-229

[10] Mineralization and toxicity reduction of the benzophenone-1 using 2D/2D Cu2WS4/BiOCl Z-scheme system: Simultaneously improved visible-light absorption and charge transfer efficiency [J].

Jiang, Runren ;

Lu, Guanghua ;

Nkoom, Matthew ;

Yan, Zhenhua ;

Wu, Donghai ;

Liu, Jianchao ;

Dang, Tianjian .

CHEMICAL ENGINEERING JOURNAL, 2020, 400

← 1 2 3 4 5 →