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Effect of Particle Aspect Ratio and Shape on the Particle-Scale Dynamics of Gas-Liquid Flow through Packed Beds
被引:4
|作者:
Ambekar, Aniket S.
[1
,2
]
Singh, Kuldeep
[1
]
Kumari, Ankita
[1
]
Buwa, Vivek V.
[1
]
机构:
[1] Indian Inst Technol Delhi, Dept Chem Engn, New Delhi 110016, India
[2] Eindhoven Univ Technol, ASA Dept Chem Engn & Chem, NL-5600 MB Eindhoven, Netherlands
关键词:
VOLUME;
REACTORS;
D O I:
10.1021/acs.iecr.3c00572
中图分类号:
TQ [化学工业];
学科分类号:
0817 ;
摘要:
Packed beds are widely used to perform solid-catalyzedgas-liquidreactions and gas cleanup processes. In the present work, we simulatedgas-liquid flow through realistic 3D particle-resolved domainsconsisting of cylindrical particles of varying aspect ratio (h = 1-5) and different particle shapes (Raschig ring,trilobe, daisy, and sphere) using the volume-of-fluid method. Withan increase in h, we found that the number fractionof laterally oriented particles decreases and length of elongatedvoid-throats increases. Further, we found that liquid preferentiallyflows over surface of laterally oriented particles and through elongatedvoid-throats. The combined effect of h, orientationdistribution, and elongated void-throats results in improved hydrodynamicperformance (liquid holdup, wetting efficiency, interfacial area,and liquid distribution) with an increase in h. Wealso found that the hydrodynamic performance of trilobe- and daisy-shapedparticles is better than cylindrical particles in terms of interfacialarea due to preferential flow of liquid through the grooves on externallyshaped particles.
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页码:18989 / 19003
页数:15
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