Quantum Sensing of Thermoelectric Power in Low-Dimensional Materials

被引:8
|
作者
Zhao, Mali [1 ,2 ]
Kim, Dohyun [2 ]
Lee, Young Hee [2 ,3 ]
Yang, Heejun [4 ]
Cho, Suyeon [5 ]
机构
[1] Tongji Univ, Coll Mat Sci & Engn, Interdisciplinary Mat Res Ctr, Shanghai 201804, Peoples R China
[2] Sungkyunkwan Univ, Dept Energy Sci, Suwon 16419, South Korea
[3] Inst Basic Sci, Ctr Integrated Nanostruct Phys CINAP, Suwon 16419, South Korea
[4] Korea Adv Inst Sci & Technol KAIST, Dept Phys, Daejeon 34141, South Korea
[5] Ewha Womans Univ, Div Chem Engn & Mat Sci, Seoul 03760, South Korea
基金
新加坡国家研究基金会;
关键词
low dimensional materials; quantum sensing; scanning probe microscopy; scanning thermoelectric microscopy; thermoelectric power; ULTRALOW THERMAL-CONDUCTIVITY; N-TYPE SNSE; BAND-GAP; THERMOPOWER; PERFORMANCE; MICROSCOPY; TRANSPORT; TEMPERATURE; SCATTERING; CHARGE;
D O I
10.1002/adma.202106871
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Thermoelectric power, has been extensively studied in low-dimensional materials where quantum confinement and spin textures can largely modulate thermopower generation. In addition to classical and macroscopic values, thermopower also varies locally over a wide range of length scales, and is fundamentally linked to electron wave functions and phonon propagation. Various experimental methods for the quantum sensing of localized thermopower have been suggested, particularly based on scanning probe microscopy. Here, critical advances in the quantum sensing of thermopower are introduced, from the atomic to the several-hundred-nanometer scales, including the unique role of low-dimensionality, defects, spins, and relativistic effects for optimized power generation. Investigating the microscopic nature of thermopower in quantum materials can provide insights useful for the design of advanced materials for future thermoelectric applications. Quantum sensing techniques for thermopower can pave the way to practical and novel energy devices for a sustainable society.
引用
收藏
页数:20
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