X-ray-to-visible light-field detection through pixelated colour conversion

被引:76
作者
Yi, Luying [1 ]
Hou, Bo [1 ]
Zhao, He [1 ,2 ,3 ]
Liu, Xiaogang [1 ,2 ,3 ,4 ,5 ]
机构
[1] Natl Univ Singapore, Dept Chem, Singapore, Singapore
[2] Natl Univ Singapore, Joint Sch, Fuzhou, Peoples R China
[3] Tianjin Univ, Fuzhou, Peoples R China
[4] Natl Univ Singapore Suzhou, Ctr Funct Mat, Res Inst, Suzhou, Peoples R China
[5] Agcy Sci Technol & Res, Inst Mat Res & Engn, Singapore, Singapore
基金
新加坡国家研究基金会;
关键词
WAVE-FRONT SENSOR; PHASE-RETRIEVAL; RESOLUTION;
D O I
10.1038/s41586-023-05978-w
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Light-field detection measures both the intensity of light rays and their precise direction in free space. However, current light-field detection techniques either require complex microlens arrays or are limited to the ultraviolet-visible light wavelength ranges(1-4). Here we present a robust, scalable method based on lithographically patterned perovskite nanocrystal arrays that can be used to determine radiation vectors from X-rays to visible light (0.002-550 nm). With these multicolour nanocrystal arrays, light rays from specific directions can be converted into pixelated colour outputs with an angular resolution of 0.0018 degrees. We find that three-dimensional light-field detection and spatial positioning of light sources are possible by modifying nanocrystal arrays with specific orientations. We also demonstrate three-dimensional object imaging and visible light and X-ray phase-contrast imaging by combining pixelated nanocrystal arrays with a colour charge-coupled device. The ability to detect light direction beyond optical wavelengths through colour-contrast encoding could enable new applications, for example, in three-dimensional phase-contrast imaging, robotics, virtual reality, tomographic biological imaging and satellite autonomous navigation.
引用
收藏
页码:281 / +
页数:8
相关论文
共 42 条
[1]   A colloidal quantum dot spectrometer [J].
Bao, Jie ;
Bawendi, Moungi G. .
NATURE, 2015, 523 (7558) :67-+
[2]   Ultrafast single-shot diffraction imaging of nanoscale dynamics [J].
Barty, Anton ;
Boutet, Sebastien ;
Bogan, Michael J. ;
Hau-Riege, Stefan ;
Marchesini, Stefano ;
Sokolowski-Tinten, Klaus ;
Stojanovic, Nikola ;
Tobey, Ra'Anan ;
Ehrke, Henri ;
Cavalleri, Andrea ;
Duesterer, Stefan ;
Frank, Matthias ;
Bajt, Sasa ;
Woods, Bruce W. ;
Seibert, M. Marvin ;
Hajdu, Janos ;
Treusch, Rolf ;
Chapman, Henry N. .
NATURE PHOTONICS, 2008, 2 (07) :415-419
[3]   X-ray pulse wavefront metrology using speckle tracking [J].
Berujon, Sebastien ;
Ziegler, Eric ;
Cloetens, Peter .
JOURNAL OF SYNCHROTRON RADIATION, 2015, 22 :886-894
[4]  
Cao LY, 2009, NAT MATER, V8, P643, DOI [10.1038/nmat2477, 10.1038/NMAT2477]
[5]   All-inorganic perovskite nanocrystal scintillators [J].
Chen, Qiushui ;
Wu, Jing ;
Ou, Xiangyu ;
Huang, Bolong ;
Almutlaq, Jawaher ;
Zhumekenov, Ayan A. ;
Guan, Xinwei ;
Han, Sanyang ;
Liang, Liangliang ;
Yi, Zhigao ;
Li, Juan ;
Xie, Xiaoji ;
Wang, Yu ;
Li, Ying ;
Fan, Dianyuan ;
Teh, Daniel B. L. ;
All, Angelo H. ;
Mohammed, Omar F. ;
Bakr, Osman M. ;
Wu, Tom ;
Bettinelli, Marco ;
Yang, Huanghao ;
Huang, Wei ;
Liu, Xiaogang .
NATURE, 2018, 561 (7721) :88-93
[6]   Continuous-wave frequency upconversion with a molecular optomechanical nanocavity [J].
Chen, Wen ;
Roelli, Philippe ;
Hu, Huatian ;
Verlekar, Sachin ;
Amirtharaj, Sakthi Priya ;
Barreda, Angela, I ;
Kippenberg, Tobias J. ;
Kovylina, Miroslavna ;
Verhagen, Ewold ;
Martinez, Alejandro ;
Galland, Christophe .
SCIENCE, 2021, 374 (6572) :1264-+
[7]   High-sensitivity high-resolution X-ray imaging with soft-sintered metal halide perovskites [J].
Deumel, Sarah ;
van Breemen, Albert ;
Gelinck, Gerwin ;
Peeters, Bart ;
Maas, Joris ;
Verbeek, Roy ;
Shanmugam, Santhosh ;
Akkerman, Hylke ;
Meulenkamp, Eric ;
Huerdler, Judith E. ;
Acharya, Manognya ;
Garcia-Batlle, Marise ;
Almora, Osbel ;
Guerrero, Antonio ;
Garcia-Belmonte, Germa ;
Heiss, Wolfgang ;
Schmidt, Oliver ;
Tedde, Sandro F. .
NATURE ELECTRONICS, 2021, 4 (09) :681-688
[8]   Video-rate imaging of biological dynamics at centimetre scale and micrometre resolution [J].
Fan, Jingtao ;
Suo, Jinli ;
Wu, Jiamin ;
Xie, Hao ;
Shen, Yibing ;
Chen, Feng ;
Wang, Guijin ;
Cao, Liangcai ;
Jin, Guofan ;
He, Quansheng ;
Li, Tianfu ;
Luan, Guoming ;
Kong, Lingjie ;
Zheng, Zhenrong ;
Dai, Qionghai .
NATURE PHOTONICS, 2019, 13 (11) :809-+
[9]  
Fan PY, 2014, NAT MATER, V13, P471, DOI [10.1038/nmat3927, 10.1038/NMAT3927]
[10]  
Gao Y, 2017, NAT PHOTONICS, V11, P301, DOI [10.1038/nphoton.2017.37, 10.1038/NPHOTON.2017.37]