Two-dimensional covalent organic frameworks for electrocatalysis: Achievements, challenges, and opportunities

被引：29
作者：
Zhao, Ruoyu [1 ]
Wang, Teng [2 ]
Li, Junjun [1 ]
Shi, Yongxia [1 ]
Hou, Man [1 ]
Yang, Yong [2 ]
Zhang, Zhicheng [1 ]
Lei, Shengbin [1 ]
机构：
[1] Tianjin Univ, Sch Sci & Tianjin Key Lab Mol Optoelect Sci, Dept Chem, Tianjin 300072, Peoples R China
[2] Northwestern Polytech Univ, Ctr Adv Lubricat & Seal Mat, State Key Lab Solidificat Proc, Xian 710072, Peoples R China
来源：
NANO RESEARCH | 2023年 / 16卷 / 07期
基金：
中国国家自然科学基金;
关键词：
covalent organic frameworks; electrocatalysts; two-dimensional; active centers; TRIAZINE-BASED FRAMEWORKS; OXYGEN-REDUCTION; EFFICIENT ELECTROCATALYST; CO2; ELECTROREDUCTION; SELECTIVE OXIDATION; FACILE SYNTHESIS; IONIC LIQUIDS; GREEN SOLVENT; ACTIVE-SITES; CRYSTALLINE;
D O I：
10.1007/s12274-022-5307-1
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Covalent organic frameworks (COFs) represent an emerging class of crystalline porous polymers with high porosity, good stability, and adjustable structure, and their excellent characteristics lay a solid foundation for electrocatalysis. This review systematically introduces the design principles of the catalytic sites in two-dimensional (2D) COF-based electrocatalysts and analyzes the relationship between 2D COF structure and their electrocatalytic performances. In particular, the recent progress in the field of 2D COFs as electrocatalysts is comprehensively summarized. Finally, we discuss the current shortcomings and challenges on tailoring 2D COF for high-performance electrocatalysts in details, and look forward to promoting more researches on 2D COF-based electrocatalysts.
引用
收藏
页码：8570 / 8595
页数：26
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