Fe- and S-Modified BiOI as Catalysts to Oxygen Evolution and Hydrogen Evolution Reactions in Overall Photoelectrochemical Water Splitting

被引：1
|
作者：
Lei, Yu [1 ,2 ]
Chen, Hongdian [2 ]
Shu, Chenyang [2 ]
Chen, Changguo [1 ]
机构：
[1] Chongqing Univ, Coll Chem & Chem Engn, Chongqing 401331, Peoples R China
[2] Chongqing Univ Arts & Sci, Chongqing Key Lab Mat Surface & Interface Sci, Chongqing 402160, Peoples R China
来源：
MATERIALS | 2024年 / 17卷 / 01期
关键词：
bismuth oxyiodide; iron modification; sulfurization; overall water splitting; photoelectrochemical catalysis; PHOTOCATALYSTS; HETEROSTRUCTURE; CONSTRUCTION; DEGRADATION; REDUCTION; COMPOSITE; REMOVAL; CLOTH;
D O I：
10.3390/ma17010006
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Developing catalysts with superior activity to hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) is equally important to the overall photoelectrochemical water splitting to produce hydrogen. In this work, bismuth oxyiodide (BiOI), iron-modified bismuth iodide Fe/BiOI, and the sulfurized S-Fe/BiOI were prepared using the solvothermal method. The three materials all have good absorption ability for visible light. The photoelectrochemical catalytic activity of BiOI to oxygen evolution reaction (OER) is significantly enhanced after iron modification, while the sulfurized product S-Fe/BiOI exhibits better catalytic activity to hydrogen evolution reaction (HER). Hence, OER and HER can be simultaneously catalyzed by using Fe/BiOI and S-Fe/BiOI as anodic and cathodic catalysts to facilitate the overall photoelectrochemical water splitting process.
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页数：12
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